Measuring the Vertical Profiles of Aerosol Extinction in the Lower Troposphere by MAX-DOAS at a Rural Site in the North China Plain

被引：5

作者：

Cheng, Siyang ^{[1
,2
]}

Jin, Junli ^{[3
]}

Ma, Jianzhong ^{[1
,2
]}

Xu, Xiaobin ^{[1
,2
]}

Ran, Liang ^{[4
]}

Ma, Zhiqiang ^{[5
]}

Chen, Junming ^{[1
,2
]}

Guo, Junrang ^{[1
,2
]}

Yang, Peng ^{[6
]}

Wang, Yang ^{[7
]}

Wagner, Thomas ^{[7
]}

机构：

[1] Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing 100081, Peoples R China

[2] Chinese Acad Meteorol Sci, CMA Key Lab Atmospher Chem, Beijing 100081, Peoples R China

[3] CMA Meteorol Observat Ctr, Beijing 100081, Peoples R China

[4] Chinese Acad Sci, Key Lab Middle Atmosphere & Global Environm Obser, Inst Atmospher Phys, Beijing 100029, Peoples R China

[5] China Meteorol Adm, Inst Urban Meteorol, Beijing 100089, Peoples R China

[6] Meteorol Bur Shijiazhuang, Shijiazhuang 050081, Hebei, Peoples R China

[7] Max Planck Inst Chem, D-55020 Mainz, Germany

来源：

ATMOSPHERE | 2020年 / 11卷 / 10期

基金：

中国国家自然科学基金;

关键词：

aerosol extinction; vertical profile; ground-based MAX-DOAS; lidar; North China plain; OPTICAL-PROPERTIES; COLUMN DENSITIES; O-4; ABSORPTIONS; NO2; RETRIEVAL; SO2; WINTER; LIDAR; HCHO; VALIDATION;

D O I：

10.3390/atmos11101037

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed during the summer (13 June-20 August) of 2014 at a rural site in North China Plain. The vertical profiles of aerosol extinction (AE) in the lower troposphere were retrieved to analyze the temporal variations of AE profiles, near-surface AE, and aerosol optical depth (AOD). The average AOD and near-surface AE over the period of study were 0.51 +/- 0.26 and 0.33 +/- 0.18 km(-1) during the effective observation period, respectively. High AE events and elevated AE layers were identified based on the time series of hourly AE profiles, near-surface AEs and AODs. It is found that in addition to the planetary boundary layer height (PBLH) and relative humidity (RH), the variations in the wind field have large impacts on the near-surface AE, AOD, and AE profile. Among 16 wind sectors, higher AOD or AE occur mostly in the directions of the cities upstream. The diurnal variations of the AE profiles, AODs and near-surface AEs are significant and influenced mainly by the source emissions, PBLH, and RH. The AE profile shape from MAX-DOAS measurement is generally in agreement with that from light detection and ranging (lidar) observations, although the AE absolute levels are different. Overall, ground-based MAX-DOAS can serve as a supplement to measure the AE vertical profiles in the lower troposphere.

引用

页数：17

共 67 条

[1] Method to retrieve aerosol extinction profiles and aerosol scattering phase functions with a modified CCD laser atmospheric detection system [J].

Bian, Y. ;

Xu, W. ;

Hu, Y. ;

Tao, J. ;

Kuang, Y. ;

Zhao, C. .

OPTICS EXPRESS, 2020, 28 (05) :6631-6647

[2] PM10 source apportionment applying PMF and chemical tracer analysis to ship-borne measurements in the Western Mediterranean [J].

Bove, M. C. ;

Brotto, P. ;

Calzolai, G. ;

Cassola, F. ;

Cavalli, F. ;

Fermo, P. ;

Hjorth, J. ;

Massabo, D. ;

Nava, S. ;

Piazzalunga, A. ;

Schembari, C. ;

Prati, P. .

ATMOSPHERIC ENVIRONMENT, 2016, 125 :140-151

[3] The 2005 and 2006 DANDELIONS NO2 and aerosol intercomparison campaigns [J].

Brinksma, E. J. ;

Pinardi, G. ;

Volten, H. ;

Braak, R. ;

Richter, A. ;

Schoenhardt, A. ;

van Roozendael, M. ;

Fayt, C. ;

Hermans, C. ;

Dirksen, R. J. ;

Vlemmix, T. ;

Berkhout, A. J. C. ;

Swart, D. P. J. ;

Oetjen, H. ;

Wittrock, F. ;

Wagner, T. ;

Ibrahim, O. W. ;

de Leeuw, G. ;

Moerman, M. ;

Curier, R. L. ;

Celarier, E. A. ;

Cede, A. ;

Knap, W. H. ;

Veefkind, J. P. ;

Eskes, H. J. ;

Allaart, M. ;

Rothe, R. ;

Piters, A. J. M. ;

Levelt, P. F. .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2008, 113 (D16)

[4] Observations of tropospheric aerosols and NO2 in Hong Kong over 5 years using ground based MAX-DOAS [J].

Chan, K. L. ;

Wiegner, M. ;

Wenig, M. ;

Poehler, D. .

SCIENCE OF THE TOTAL ENVIRONMENT, 2018, 619 :1545-1556

[5] Ground-based aerosol climatology of China: aerosol optical depths from the China Aerosol Remote Sensing Network (CARSNET) 2002-2013 [J].

Che, H. ;

Zhang, X. -Y. ;

Xia, X. ;

Goloub, P. ;

Holben, B. ;

Zhao, H. ;

Wang, Y. ;

Zhang, X. -C. ;

Wang, H. ;

Blarel, L. ;

Damiri, B. ;

Zhang, R. ;

Deng, X. ;

Ma, Y. ;

Wang, T. ;

Geng, F. ;

Qi, B. ;

Zhu, J. ;

Yu, J. ;

Chen, Q. ;

Shi, G. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2015, 15 (13) :7619-7652

[6] Column aerosol optical properties and aerosol radiative forcing during a serious haze-fog month over North China Plain in 2013 based on ground-based sunphotometer measurements [J].

Che, H. ;

Xia, X. ;

Zhu, J. ;

Li, Z. ;

Dubovik, O. ;

Holben, B. ;

Goloub, P. ;

Chen, H. ;

Estelles, V. ;

Cuevas-Agullo, E. ;

Blarel, L. ;

Wang, H. ;

Zhao, H. ;

Zhang, X. ;

Wang, Y. ;

Sun, J. ;

Tao, R. ;

Zhang, X. ;

Shi, G. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2014, 14 (04) :2125-2138

[7] Spatial distribution of aerosol microphysical and optical properties and direct radiative effect from the China Aerosol Remote Sensing Network [J].

Che, Huizheng ;

Xia, Xiangao ;

Zhao, Hujia ;

Dubovik, Oleg ;

Holben, Brent N. ;

Goloub, Philippe ;

Cuevas-Agullo, Emilio ;

Estelles, Victor ;

Wang, Yaqiang ;

Zhu, Jun ;

Qi, Bing ;

Gong, Wei ;

Yang, Honglong ;

Zhang, Renjian ;

Yang, Leiku ;

Chen, Jing ;

Wang, Hong ;

Zheng, Yu ;

Gui, Ke ;

Zhang, Xiaochun ;

Zhang, Xiaoye .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (18) :11843-11864

[8] Long-term validation of MODIS C6 and C6.1 Dark Target aerosol products over China using CARSNET and AERONET [J].

Che, Huizheng ;

Yang, Leiku ;

Liu, Chao ;

Xia, Xiangao ;

Wang, Yaqiang ;

Wang, Hong ;

Wang, Han ;

Lu, Xiaofeng ;

Zhang, Xiaoye .

CHEMOSPHERE, 2019, 236

[9] A synchronous observation of enhanced aerosol and NO2 over Beijing, China, in winter 2015 [J].

Chen, Zhenyi ;

Liu, Cheng ;

Liu, Wenqing ;

Zhang, Tianshu ;

Xu, Jin .

SCIENCE OF THE TOTAL ENVIRONMENT, 2017, 575 :429-436

[10] Tropospheric NO2 vertical column densities retrieved from ground-based MAX-DOAS measurements at Shangdianzi regional atmospheric background station in China [J].

Cheng, Siyang ;

Ma, Jianzhong ;

Cheng, Weiping ;

Yan, Peng ;

Zhou, Huaigang ;

Zhou, Liyan ;

Yang, Peng .

JOURNAL OF ENVIRONMENTAL SCIENCES, 2019, 80 :186-196

← 1 2 3 4 5 6 7 →