Investigation of giant magnetoconductance in organic devices based on hopping mechanism

被引:13
作者
Yang, F. J. [1 ]
Qin, W. [1 ]
Xie, S. J. [1 ]
机构
[1] Shandong Univ, Sch Phys, State Key Lab Crystal Mat, Jinan 250100, Peoples R China
关键词
LIGHT-EMITTING-DIODES; ROOM-TEMPERATURE; SEMICONDUCTING MATERIALS; CONJUGATED POLYMERS; ELECTRON-MOBILITY; MAGNETORESISTANCE; FILMS;
D O I
10.1063/1.4869936
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We suggest a spin-dependent hopping mechanism which includes the effect of the external magnetic field as well as hyperfine interaction (HFI) to explain the observed giant magnetoconductance (MC) in non-magnetic organic devices. Based on the extended Marcus theory, we calculate the MC by using the master equation. It is found that a MC value as large as 91% is obtained under a low driving voltage. For suitable parameters, the theoretical results are in good agreement with the experimental data. Influences of the carrier density, HFI, and the carrier localization on the MC value are investigated. Especially, it is found that a low-dimensional structure of the organic materials is favorable to get a large MC value. (C) 2014 AIP Publishing LLC.
引用
收藏
页数:5
相关论文
共 32 条
[1]   Hopping Magnetotransport via Nonzero Orbital Momentum States and Organic Magnetoresistance [J].
Alexandrov, Alexandre S. ;
Dediu, Valentin A. ;
Kabanov, Victor V. .
PHYSICAL REVIEW LETTERS, 2012, 108 (18)
[2]   Electron mobility in tris(8-hydroxy-quinoline)aluminum thin films determined via transient electroluminescence from single- and multilayer organic light-emitting diodes [J].
Barth, S ;
Müller, P ;
Riel, H ;
Seidler, PF ;
Riess, W ;
Vestweber, H ;
Bässler, H .
JOURNAL OF APPLIED PHYSICS, 2001, 89 (07) :3711-3719
[3]   Bipolaron mechanism for organic magnetoresistance [J].
Bobbert, P. A. ;
Nguyen, T. D. ;
van Oost, F. W. A. ;
Koopmans, B. ;
Wohlgenannt, M. .
PHYSICAL REVIEW LETTERS, 2007, 99 (21)
[4]   Challenges for organic spintronics [J].
Boehme, Christoph ;
Lupton, John M. .
NATURE NANOTECHNOLOGY, 2013, 8 (09) :612-615
[5]   Large magnetic field effects in organic light emitting diodes based on tris(8-hydroxyquinoline aluminum) (Alq3)/IN,N′-Di(naphthalen-1-yl)-N,N′ diphenyl-benzidine (NPB) bilayers [J].
Davis, AH ;
Bussmann, K .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A, 2004, 22 (04) :1885-1891
[6]   Magnetoresistance in organic light-emitting diode structures under illumination [J].
Desai, P. ;
Shakya, P. ;
Kreouzis, T. ;
Gillin, W. P. .
PHYSICAL REVIEW B, 2007, 76 (23)
[7]   Magnetoresistance and efficiency measurements of Alq3-based OLEDs [J].
Desai, Pratik ;
Shakya, P. ;
Kreouzis, T. ;
Gillin, W. P. ;
Morley, N. A. ;
Gibbs, M. R. J. .
PHYSICAL REVIEW B, 2007, 75 (09)
[8]   Magnetic field effects on the electroluminescence of organic light emitting devices: A tool to indicate the carrier mobility [J].
Ding, B. F. ;
Yao, Y. ;
Sun, Z. Y. ;
Wu, C. Q. ;
Gao, X. D. ;
Wang, Z. J. ;
Ding, X. M. ;
Choy, W. C. H. ;
Hou, X. Y. .
APPLIED PHYSICS LETTERS, 2010, 97 (16)
[9]   Large magnetoresistance at room temperature in semiconducting polymer sandwich devices -: art. no. 185 [J].
Francis, TL ;
Mermer, Ö ;
Veeraraghavan, G ;
Wohlgenannt, M .
NEW JOURNAL OF PHYSICS, 2004, 6 :1-8
[10]   Molecular origin of differences in hole and electron mobility in amorphous Alq3-a multiscale simulation study [J].
Fuchs, Andreas ;
Steinbrecher, Thomas ;
Mommer, Mario S. ;
Nagata, Yuki ;
Elstner, Marcus ;
Lennartz, Christian .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2012, 14 (12) :4259-4270