Enhanced visible-light-induced photocatalytic degradation of tetracycline using BiOI/MIL-125(Ti) composite photocatalyst

被引:151
作者
Jiang, Wei [1 ,2 ]
Li, Zhi [2 ]
Liu, Chunbo [1 ,2 ]
Wang, Dandan [1 ,2 ]
Yan, Guosong [1 ]
Liu, Bo [1 ]
Che, Guangbo [1 ]
机构
[1] Jilin Normal Univ, Minist Educ, Key Lab Preparat & Applicat Environm Friendly Mat, Changchun 130103, Peoples R China
[2] Jilin Normal Univ, Coll Environm Sci & Engn, Siping 136000, Peoples R China
基金
中国国家自然科学基金;
关键词
BiOI; MOF; Photocatalyst; Tetracycline degradation;
D O I
10.1016/j.jallcom.2020.157166
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Herein, coupling semiconductor with metal-organic framework, a series of BiOI/MIL-125(Ti) composites have been prepared via one-step hydrothermal method. Morphology analyses reveal that the formation of heterostructure and the BiOI is uniformly covering on the surface of MIL-125(Ti). Under visible light illumination, the optimized 9 wt% BiOI/MIL-125(Ti) composite (BT-9) exhibits excellent photocatalytic activity for the degradation of tetracycline (TC) and the efficiency could reach 80%, which is much higher than that of bare BiOI and MIL-125(Ti). In particular, the BT-9 photocatalyst features superior stability and reusability in successive catalytic runs. Based on the comprehensive characterization studies, the enhancement of photocatalytic activity can be ascribed to the high specific surface area, promoting visible light absorption and outstanding efficiency of charge transfer of BiOI/MIL-125(Ti) composites. (C) 2020 Elsevier B.V. All rights reserved.
引用
收藏
页数:10
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