The synthesis of a hierarchically porous BEA zeolite via pseudomorphic crystallization

被引:82
作者
Choi, Minkee [1 ]
Na, Kyungsu [1 ]
Ryoo, Ryong [1 ]
机构
[1] Korea Adv Inst Sci & Technol, Dept Chem, Grad Sch Nanosci & Technol WCU, Ctr Funct Nanomat, Taejon 305701, South Korea
关键词
DRY-GEL CONVERSION; ZSM-5; MESOPOROSITY; DESILICATION; GENERATION; STABILITY; MECHANISM; CRYSTALS; CATIONS; BETA;
D O I
10.1039/b905087f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A synthesis route to a hierarchically meso-/microporous BEA zeolite has been developed with a cyclic diammonium as a structure-directing agent (SDA), which leads to pseudomorphic crystallization of the zeolite by suppressing the mobility of silicates during crystallization.
引用
收藏
页码:2845 / 2847
页数:3
相关论文
共 31 条
[1]  
Anderson MW, 2000, ANGEW CHEM INT EDIT, V39, P2707, DOI 10.1002/1521-3773(20000804)39:15<2707::AID-ANIE2707>3.0.CO
[2]  
2-M
[3]   CRYSTALLIZATION OF ZEOLITE BETA - EFFECT OF NA AND K-IONS [J].
CAMBLOR, MA ;
PEREZPARIENTE, J .
ZEOLITES, 1991, 11 (03) :202-210
[4]   Amphiphilic organosilane-directed synthesis of crystalline zeolite with tunable mesoporosity [J].
Choi, Minkee ;
Cho, Hae Sung ;
Srivastava, Rajendra ;
Venkatesan, Chithravel ;
Choi, Dae-Heung ;
Ryoo, Ryong .
NATURE MATERIALS, 2006, 5 (09) :718-723
[5]   SHAPE-SELECTIVE ALKYLATION OF NAPHTHALENE WITH ISOPROPANOL OVER LARGE-PORE ZEOLITES [J].
CHU, SJ ;
CHEN, YW .
APPLIED CATALYSIS A-GENERAL, 1995, 123 (01) :51-58
[6]   The hydrothermal synthesis of zeolites: Precursors, intermediates and reaction mechanism [J].
Cundy, CS ;
Cox, PA .
MICROPOROUS AND MESOPOROUS MATERIALS, 2005, 82 (1-2) :1-78
[7]   Templating mesoporous zeolites [J].
Egeblad, Kresten ;
Christensen, Christina H. ;
Kustova, Marina ;
Christensen, Claus H. .
CHEMISTRY OF MATERIALS, 2008, 20 (03) :946-960
[8]  
GANG L, 1999, APPL CATAL A-GEN, V185, P11
[9]   Direct demonstration of enhanced diffusion in mesoporous ZSM-5 zeolite obtained via controlled desilication [J].
Groen, Johan C. ;
Zhu, Weidong ;
Brouwer, Sander ;
Huynink, Steven J. ;
Kapteijn, Freek ;
Moulijn, Jacob A. ;
Perez-Ramirez, Javier .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (02) :355-360
[10]   Desilication:: on the controlled generation of mesoporosity in MFI zeolites [J].
Groen, Johan C. ;
Moulijn, Jacob A. ;
Perez-Ramirez, Javier .
JOURNAL OF MATERIALS CHEMISTRY, 2006, 16 (22) :2121-2131