Distribution of 127I and 129I in precipitation at high European latitudes

被引:40
作者
Aldahan, A. [1 ,2 ]
Persson, S. [3 ]
Possnert, G. [3 ]
Hou, X. L. [4 ,5 ]
机构
[1] Uppsala Univ, Dept Earth Sci, SE-75836 Uppsala, Sweden
[2] United Arab Emirates Univ, Dept Geol, Al Ain, U Arab Emirates
[3] Uppsala Univ, Tandem Lab, SE-75121 Uppsala, Sweden
[4] Tech Univ Denmark, Riso Natl Lab Sustainable Energy, DK-4000 Roskilde, Denmark
[5] CAS, Inst Earth Environm, SKLLQG, Xian, Peoples R China
关键词
PARTICLE FORMATION; IODINE EMISSIONS; MOLECULAR-IODINE; METHYL-IODIDE; BALTIC SEA; NORTH-SEA; SPECIATION; SEAWATER; TRANSECT; AEROSOL;
D O I
10.1029/2009GL037363
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
We here present the most extensive data set on the distribution of I-127 and I-129 in precipitation (rain and snow) covering the period 2000-2006 and European latitudes 55 degrees N-68 degrees N. Our results indicate a wide variation in the concentrations and fluxes of the two isotopes associated with generally higher values at near coastal sites compared to the inland ones. Total wet-related annual deposition of I-127 and I-129 on Sweden and Denmark is estimated at about 1.2 x 10(9) g and 60 g respectively. The average annual I-129 wet deposition accounts for <1% and <0.05% of the total annual gaseous and liquid, respectively, discharges from the Sellafiled and La Hague Facilities. The I-127 annual wet deposition represents < 1% of the estimated global oceanic iodine flux. Air mass trajectories suggest that events of enhanced I-129 in precipitation are closely related to southwesterly weather fronts from regions of elevated concentrations. Citation: Aldahan, A., S. Persson, G. Possnert, and X. L. Hou (2009), Distribution of I-127 and I-129 in precipitation at high European latitudes, Geophys. Res. Lett., 36, L11805, doi: 10.1029/2009GL037363.
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页数:5
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