Numerical analysis on the power consumption of the PSA process for recovering CO2 from flue gas

被引:97
作者
Park, JH [1 ]
Beum, HT [1 ]
Kim, JN [1 ]
Cho, SH [1 ]
机构
[1] Korea Inst Energy Res, Yusungku, Taejon 305343, South Korea
关键词
D O I
10.1021/ie010716i
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
To recover 99% CO2 from flue gas containing 10-15% CO2, a two-stage pressure swing adsorption (PSA) process is usually employed. At the first stage of the two-stage PSA, CO2 is concentrated to 40-60% and then concentrated to 99% at the second stage. Because two stages are coupled with each other, the overall optimization of the two-stage PSA process is quite a complicated task. In this paper, we only considered the first stage of the two-stage PSA process to simplify the analysis. Effects of the process configuration and operating variables such as the P/F ratio and desorption pressure on the specific power consumption were investigated. The specific power consumption at the blower was reduced with the increase of the P/F ratio. On the contrary, that at the vacuum pump was increased with the increase of the P/F ratio. Because of these two effects, there was an optimum PIF ratio, which minimized the specific power consumption. While the compression ratio is reduced with the increase of the desorption pressure, the CO2 purity is decreased and the amount of the power used to compress nitrogen is increased. As a result, the specific power consumption was insensitive to the desorption pressure within the range studied here. Employing the pressure equalization step, the CO2 purity could be increased without much increase of the specific power consumption. With the rinse step, which is often used to increase the purity of the strongly adsorbed component, the CO2 purity could be increased. However, because more gases should be pumped to produce a given amount of CO2, the specific power consumption was significantly increased at a given recovery.
引用
收藏
页码:4122 / 4131
页数:10
相关论文
共 14 条
[1]   A NEW COMPOSITE SORBENT FOR METHANE-NITROGEN SEPARATION BY ADSORPTION [J].
BAKSH, MSA ;
KAPOOR, A ;
YANG, RT .
SEPARATION SCIENCE AND TECHNOLOGY, 1990, 25 (7-8) :845-868
[2]   SEPARATION OF BINARY GAS-MIXTURE INTO 2 HIGH-PURITY PRODUCTS BY A NEW PRESSURE SWING ADSORPTION CYCLE [J].
CEN, PL ;
YANG, RT .
SEPARATION SCIENCE AND TECHNOLOGY, 1986, 21 (09) :845-864
[3]   COMPARISON OF ACTIVATED CARBON AND ZEOLITE 13X FOR CO2 RECOVERY FROM FLUE-GAS BY PRESSURE SWING ADSORPTION [J].
CHUE, KT ;
KIM, JN ;
YOO, YJ ;
CHO, SH ;
YANG, RT .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1995, 34 (02) :591-598
[4]   NEW PSA PROCESS WITH INTERMEDIATE FEED INLET POSITION OPERATED WITH DUAL REFLUXES - APPLICATION TO CARBON-DIOXIDE REMOVAL AND ENRICHMENT [J].
DIAGNE, D ;
GOTO, M ;
HIROSE, T .
JOURNAL OF CHEMICAL ENGINEERING OF JAPAN, 1994, 27 (01) :85-89
[5]   PARAMETRIC STUDIES ON CO2 SEPARATION AND RECOVERY BY A DUAL REFLUX PSA PROCESS CONSISTING OF BOTH RECTIFYING AND STRIPPING SECTIONS [J].
DIAGNE, D ;
GOTO, M ;
HIROSE, T .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1995, 34 (09) :3083-3089
[6]   Technology for removing carbon dioxide from power plant flue gas by the physical adsorption method [J].
Ishibashi, M ;
Ota, H ;
Akutsu, N ;
Umeda, S ;
Tajika, M ;
Izumi, J ;
Yasutake, A ;
Kabata, T ;
Kageyama, Y .
ENERGY CONVERSION AND MANAGEMENT, 1996, 37 (6-8) :929-933
[7]   KINETIC SEPARATION OF METHANE CARBON-DIOXIDE MIXTURE BY ADSORPTION ON MOLECULAR-SIEVE CARBON [J].
KAPOOR, A ;
YANG, RT .
CHEMICAL ENGINEERING SCIENCE, 1989, 44 (08) :1723-1733
[8]   CONCENTRATION AND RECOVERY OF CO2 FROM FLUE-GAS BY PRESSURE SWING ADSORPTION [J].
KIKKINIDES, ES ;
YANG, RT ;
CHO, SH .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1993, 32 (11) :2714-2720
[9]   NONISOTHERMAL ADSORPTION OF NITROGEN-CARBON DIOXIDE MIXTURE IN A FIXED-BED OF ZEOLITE-X [J].
KIM, JN ;
CHUE, KT ;
KIM, KI ;
CHO, SH ;
KIM, JD .
JOURNAL OF CHEMICAL ENGINEERING OF JAPAN, 1994, 27 (01) :45-51
[10]  
KIM JN, 1994, THESIS KAIST KOREA