Porous and three dimensional titanium nitride supported platinum as an electrocatalyst for oxygen reduction reaction

被引：50

作者：

Zheng, Yuying ^{[1
]}

Zhang, Jian ^{[1
]}

Zhan, Hengtong ^{[1
]}

Sun, Dalei ^{[1
]}

Dang, Dai ^{[1
]}

Tian, Xin Long ^{[2
]}

机构：

[1] Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China

[2] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, 1037 Luoyu Rd, Wuhan 430074, Hubei, Peoples R China

来源：

ELECTROCHEMISTRY COMMUNICATIONS | 2018年 / 91卷

基金：

中国博士后科学基金;

关键词：

Transition metal nitrides; Hierarchical; Oxygen reduction reaction; Durability; Three dimensional; METHANOL OXIDATION REACTION; HIGHLY STABLE ELECTROCATALYSTS; TEMPERATURE FUEL-CELLS; PT-BASED CATALYSTS; HIGH-PERFORMANCE; NANOPARTICLES; NANOCRYSTALS; DURABILITY; NANOTUBES; LAYER;

D O I：

10.1016/j.elecom.2018.04.021

中图分类号：

O646 [电化学、电解、磁化学];

学科分类号：

081704 ;

摘要：

The development of a catalyst that is both effective and robust is desirable, but remains a challenge for those aiming to commercialize polymer electrolyte membrane fuel cells. Thus, a facile method is proposed to develop hierarchical and three-dimensional titanium nitride (TiN) architectures, with the robust non-carbon material being implemented as the Pt support. The resulting catalyst (Pt/TiN) demonstrates high activity and stability, and the experimental data confirm the critical significance of the novel TiN support.

引用

页码：31 / 35

页数：5

共 34 条

[1] Highly Crystalline Multimetallic Nanoframes with Three-Dimensional Electrocatalytic Surfaces [J].

Chen, Chen ;

Kang, Yijin ;

Huo, Ziyang ;

Zhu, Zhongwei ;

Huang, Wenyu ;

Xin, Huolin L. ;

Snyder, Joshua D. ;

Li, Dongguo ;

Herron, Jeffrey A. ;

Mavrikakis, Manos ;

Chi, Miaofang ;

More, Karren L. ;

Li, Yadong ;

Markovic, Nenad M. ;

Somorjai, Gabor A. ;

Yang, Peidong ;

Stamenkovic, Vojislav R. .

SCIENCE, 2014, 343 (6177) :1339-1343

[2] Mesoporous Ti0.5Nb0.5N Ternary Nitride as a Novel Noncarbon Support for Oxygen Reduction Reaction in Acid and Alkaline Electrolytes [J].

Cui, Zhiming ;

Burns, Raymond G. ;

DiSalvo, Francis J. .

CHEMISTRY OF MATERIALS, 2013, 25 (19) :3782-3784

[3] High-Performance, Ultra low Platinum Membrane Electrode Assembly Fabricated by In Situ Deposition of a Pt Shell Layer on Carbon-Supported Pd Nanoparticles in the Catalyst Layer Using a Facile Pulse Electrodeposition Approach [J].

Dang, Dai ;

Zou, Haobin ;

Xiong, Zi'ang ;

Hou, Sanying ;

Shu, Ting ;

Nan, Haoxiong ;

Zeng, Xiaoyuan ;

Zeng, Jianhuang ;

Liao, Shijun .

ACS CATALYSIS, 2015, 5 (07) :4318-4324

[4] Electrocatalysis on Shape-Controlled Titanium Nitride Nanocrystals for the Oxygen Reduction Reaction [J].

Dong, Youzhen ;

Wu, Yongmin ;

Liu, Mengjia ;

Li, Jinghong .

CHEMSUSCHEM, 2013, 6 (10) :2016-2021

[5] Embedding Pt Nanocrystals in N-Doped Porous Carbon/Carbon Nanotubes toward Highly Stable Electrocatalysts for the Oxygen Reduction Reaction [J].

Guo, Lin ;

Jiang, Wen-Jie ;

Zhang, Yun ;

Hu, Jin-Song ;

Wei, Zi-Dong ;

Wan, Li-Jun .

ACS CATALYSIS, 2015, 5 (05) :2903-2909

[6] Titanium nitride-carbon nanotube core-shell composites as effective electrocatalyst supports for low temperature fuel cells [J].

Higgins, Drew C. ;

Choi, Ja-Yeon ;

Wu, Jason ;

Lopez, Anand ;

Chen, Zhongwei .

JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (09) :3727-3732

[7] The effect of Mn addition on the promotion of oxygen reduction reaction performance for PtCo/C catalysts [J].

Hsu, Shu-Ping ;

Liu, Chen-Wei ;

Chen, Hong-Shuo ;

Chen, Tsan-Yao ;

Lai, Chien-Ming ;

Lee, Chih-Hao ;

Lee, Jyh-Fu ;

Chan, Ting-Shan ;

Tsai, Li-Duan ;

Wang, Kuan-Wen .

ELECTROCHIMICA ACTA, 2013, 105 :180-187

[8] Increasing Pt oxygen reduction reaction activity and durability with a carbon-doped TiO2 nanocoating catalyst support [J].

Huang, Kan ;

Sasaki, Kotaro ;

Adzic, Radoslav R. ;

Xing, Yangchuan .

JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (33) :16824-16832

[9] Electrocatalytic Activity and Stability of Titania-Supported Platinum-Palladium Electrocatalysts for Polymer Electrolyte Membrane Fuel Cell [J].

Huang, Sheng-Yang ;

Ganesan, Prabhu ;

Popov, Branko N. .

ACS CATALYSIS, 2012, 2 (05) :825-831

[10] Nitride Stabilized PtNi Core-Shell Nanocatalyst for high Oxygen Reduction Activity [J].

Kuttiyiel, Kurian A. ;

Sasaki, Kotaro ;

Choi, YongMan ;

Su, Dong ;

Liu, Ping ;

Adzic, Radoslav R. .

NANO LETTERS, 2012, 12 (12) :6266-6271

← 1 2 3 4 →