Versatility of a Nitrogen-Containing Monolithic Porous Carbon for Lithium-Based Energy Storage

被引：3

作者：

Tesio, Alvaro Y. ^{[1
]}

Arias, Analia N. ^{[2
]}

Morales, Julian ^{[3
]}

Planes, Gabriel A. ^{[1
]}

Caballero, Alvaro ^{[3
]}

机构：

[1] Univ Nacl Rio Cuarto, Dept Quim, Fac Ciencias Exactas Fis Quim & Nat, Ruta Nac 36 Km 601, Cordoba, Argentina

[2] Univ Nacl Jujuy, Ctr Invest & Desarrollo Mat Avanzados & Almacenam, CONICET, Ctr Desarrollo Tecnol Gen Savio, Papala, Jujuy, Argentina

[3] Univ Cordoba, Dept Quim Inorgan, Inst Univ Invest Quim Fina & Nanoquim, Campus Rabanales, E-14071 Cordoba, Spain

来源：

CHEMISTRYSELECT | 2018年 / 3卷 / 29期

关键词：

Energy storage; Lithium batteries; Monolithic Nitrogen-containing carbon; Sulfur cathodes; DOPED MESOPOROUS CARBON; OXYGEN REDUCTION REACTION; LI-S BATTERIES; CO2; CAPTURE; GRAPHENE; FORMALDEHYDE; PERFORMANCE; ELECTRODES; RESORCINOL; CATALYSTS;

D O I：

10.1002/slct.201801330

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

N-containing monolithic porous carbon material with dual micro and mesoporous structures was synthesized using an innovative, cheap and easy synthesis route based on the classical resorcinol-formaldehyde synthesis. A completely chemical, structural and morphological characterization was carried out. The N content in the carbonaceous material was 7.3% and XPS data showed that is present in two different surrounds, as N-pyrrolic and N-pyridinic atoms. Is known that, the last one, can acts as a catalyst at surface level in heterogeneous reactions. In addition, using this material, we were able to fabricate lithium-ion and lithium-sulfur batteries obtaining high values of discharge capacity and cycle stability and demonstrating the multifunctional character of this carbon in energy storage devices.

引用

页码：8560 / 8567

页数：8

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