Electricity generation from phase-engineered flexible MoS2 nanosheets under moisture

被引:74
作者
He, Dunren [1 ,2 ]
Yang, Yaocheng [1 ,2 ]
Zhou, Yuan [1 ,2 ]
Wan, Juanyong [1 ,2 ]
Wang, Heao [1 ,2 ]
Fan, Xi [3 ]
Li, Qi [4 ]
Huang, Huihui [1 ,2 ]
机构
[1] Hunan Univ, Sch Phys & Elect, Key Lab Micro Nano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China
[2] Hunan Univ, Sch Phys & Elect, Hunan Prov Key Lab Low Dimens Struct Phys & Devic, Changsha 410082, Hunan, Peoples R China
[3] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China
[4] Shenzhen Lubon Technol Co Ltd, Shenzhen 518000, Peoples R China
基金
中国国家自然科学基金;
关键词
Hydroelectricity; Phase-engineered; Flexible; Transition metal dichalcogenides; Hydrovoltaic effect;
D O I
10.1016/j.nanoen.2020.105630
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Hydroelectricity is an emerging novel electricity generation phenomenon that the hydrogen bond energy is converted into chemical potential energy as electric power source by absorbing moisture. Here we report a high-performance water vapour energy harvester based on flexible MoS2 nanosheets with a phase gradient from 1T to 2H. The phase-engineered MoS2 film could provide open-circuit voltage and short-circuit current output of 19 mV and 6.24 mu A with a low internal resistance of 3 k Omega. Additionally, the underlying mechanism of electricity generation from phase-engineered MoS2 films was proposed in terms of contrast experiments and the plane wave density functional theory (DFT). Because of the advantages like flexible, safe, light weight and ease of scale production, this novel hydrovoltaic device could be designed as self-powered human-breathing monitor that can be integrated in disposable masks. The output voltage can be further enhanced to power commercial electronic devices by the serial connections of phase-engineered MoS2 sponges.
引用
收藏
页数:8
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