Efficient Third Harmonic Generation from Metal-Dielectric Hybrid Nanoantennas

被引:220
作者
Shibanuma, Toshihiko [1 ,2 ]
Grinblat, Gustavo [1 ]
Albella, Pablo [1 ,3 ]
Maier, Stefan A. [1 ]
机构
[1] Imperial Coll London, Dept Phys, Blackett Lab, London SW7 2AZ, England
[2] JX Nippon Oil & Energy Corp, Cent Tech Res Lab, Naka Ku, 8 Chidori Cho, Yokohama, Kanagawa 2310815, Japan
[3] Univ Las Palmas Gran Canaria, Univ Inst Intelligent Syst & Numer Applicat Engn, Las Palmas Gran Canaria 35017, Spain
基金
英国工程与自然科学研究理事会;
关键词
Metal-dielectric hybrid nanoantennas; third harmonic generation; electric field enhancement; anapole modes; SURFACE-ENHANCED SPECTROSCOPIES; 3RD-HARMONIC GENERATION; NANOPARTICLES DRIVEN; GOLD NANOPARTICLES; MAGNETIC RESPONSE; FANO RESONANCES; ANAPOLE MODES; METAMATERIALS; PLASMONICS; SCATTERING;
D O I
10.1021/acs.nanolett.7b00462
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
High refractive index dielectric nanoantennas are expected to become key elements for nonlinear nano-optics applications due to their large nonlinearities, low energy losses, and ability to produce high electric field enhancements in relatively large nanoscale volumes. In this work, we show that the nonlinear response from a high-index dielectric nanoantenna can be significantly improved by adding a metallic component to build a metal-dielectric hybrid nanostructure. We demonstrate that the plasmonic resonance of a Au nanoring can boost the anapole mode supported by a Si nanodisk, strongly enhancing the electric field inside the large third-order susceptibility dielectric. As a result, a high third harmonic conversion efficiency, which reaches 0.007% at a third harmonic wavelength of 440 nm, is obtained. In addition, by suitably modifying geometrical parameters of the hybrid nanoantenna, we tune the enhanced third harmonic emission throughout the optical regime. Coupling metallic and dielectric nanoantennas to expand the potential of subwavelength structures opens new paths for efficient nonlinear optical effects in the visible range on the nanoscale.
引用
收藏
页码:2647 / 2651
页数:5
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