Bound electronic and free carrier nonlinearities in Silicon nanocrystals at 1550nm

被引:78
作者
Spano, R. [1 ]
Daldosso, N. [1 ]
Cazzanelli, M. [1 ]
Ferraioli, L. [1 ]
Tartara, L. [3 ]
Yu, J. [3 ]
Degiorgio, V. [3 ]
Jordana, E. [2 ]
Fedeli, J. M. [2 ]
Pavesi, L. [1 ]
机构
[1] Univ Trent, Dipartimento Fis, Nanosci Lab, I-38050 Povo, Italy
[2] CEA LETI, F-38054 Grenoble 9, France
[3] Univ Pavia, Dipartimento Elettron, I-27100 Pavia, Italy
关键词
OPTICAL NONLINEARITIES;
D O I
10.1364/OE.17.003941
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present a detailed investigation of the different processes responsible for the optical nonlinearities of silicon nanocrystals at 1550 nm. Through z-scan measurements, the bound-electronic and excited carrier contributions to the nonlinear refraction were measured in presence of two-photon absorption. A study of the nonlinear response at different excitation powers has permitted to determine the change in the refractive index per unit of photo-excited carrier density sigma(r) and the value of the real bound-electronic nonlinear refraction n(2be) as a function of the nanocrystals size. Moreover at high excitation power, a saturation of the nonlinear absorption was observed due to band-filling effects. (C) 2009 Optical Society of America
引用
收藏
页码:3941 / 3950
页数:10
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