Two-dimensional electronic spectroscopy with active phase Management†

被引：0

作者：

Zhu, Wei-da ^{[1
,2
]}

Wang, Rui ^{[1
,2
]}

Wang, Xiao-yong ^{[1
,2
]}

Xiao, Min ^{[1
,2
,3
]}

Zhang, Chun-feng ^{[1
,2
]}

机构：

[1] Nanjing Univ, Natl Lab Solid State Microstruct, Sch Phys, Nanjing 210093, Peoples R China

[2] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China

[3] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA

来源：

CHINESE JOURNAL OF CHEMICAL PHYSICS | 2021年 / 34卷 / 01期

基金：

国家重点研发计划; 中国国家自然科学基金;

关键词：

Two-dimensional electronic spectroscopy; Active phase management; Frequency comb;

D O I：

10.1063/1674-0068/cjcp2012222

中图分类号：

O64 [物理化学（理论化学）、化学物理学]; O56 [分子物理学、原子物理学];

学科分类号：

070203 ; 070304 ; 081704 ; 1406 ;

摘要：

Two-dimensional electronic spectroscopy (2DES) is a powerful method to probe the coherent electron dynamics in complicated systems. Stabilizing the phase difference of the incident ultrashort pulses is the most challenging part for experimental demonstration of 2DES. Here, we present a tutorial review on the 2DES protocols based on active phase managements which are originally developed for quantum optics experiments. We introduce the 2DES techniques in box and pump-probe geometries with phase stabilization realized by interferometry, and outline the fully collinear 2DES approach with the frequency tagging by acoustic optical modulators and frequency combs. The combination of active phase managements, ultrashort pulses and other spectroscopic methods may open new opportunities to tackle essential challenges related to excited states.

引用

页码：30 / 42

页数：13

共 88 条

[1] Coherent Multidimensional Optical Spectroscopy of Excitons in Molecular Aggregates; Quasiparticle versus Supermolecule Perspectives [J].