Scintillation properties of Gd3(Al5-xGax)O12:Ce (x=2.3, 2.6, 3.0) single crystals

被引:18
作者
Chewpraditkul, Warut [1 ]
Pattanaboonmee, Nakarin [1 ]
Sakthong, Ongsa [1 ]
Chewpraditkul, Weerapong [1 ]
Szczesniak, Tomasz [2 ]
Moszynski, Marek [2 ]
Kamada, Kei [3 ,4 ]
Kurosawa, Shunsuke [3 ,4 ]
Yoshikawa, Akira [3 ,4 ]
Nikl, Martin [5 ]
机构
[1] King Mongkuts Univ Technol Thonburi, Bangkok 10140, Thailand
[2] Natl Ctr Nucl Res, A Soltana 7, PL-05400 Otwock, Poland
[3] Tohoku Univ, IMR, Sendai, Miyagi 9808577, Japan
[4] Tohoku Univ, New Ind Creat Hatchery Ctr NICHe, Sendai, Miyagi 9808579, Japan
[5] ASCR, Inst Phys, Cukrovarnicka 10, Prague 16253, Czech Republic
基金
欧盟地平线“2020”;
关键词
Energy resolution; Gd-3(Al; Ga)(5)O-12:Ce; Light yield; Nonproportionality of light yield; Scintillation decay; Coincidence time resolution; OPTICAL-PROPERTIES; ENERGY RESOLUTION; GARNET; LUMINESCENCE; GA; AL; PERFORMANCE; GROWTH; RATIO; CE3+;
D O I
10.1016/j.optmat.2018.05.015
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Scintillation properties of Czochralski-grown Gd-3(Al5-xGax)O-12:Ce (x = 2.3, 2.6, 3.0) single crystals were investigated. With increasing Ga content in garnet host, the radioluminescence band due to 5d(1)-> 4f emission transition was blue-shifted due to a decrease in the crystal field splitting of the 5 d levels. At 662 keV gamma rays, the LY value of 47,000, 55,100 and 51,900 ph/MeV was obtained for Gd3Al2.7Ga2.3O12:Ce, Gd3Al2.4Ga2.6O12:Ce and Gd3Al2Ga3O12:Ce, respectively. In spite of a lower LY value, Gd3Al2.7Ga2.3O12:Ce shows good energy resolution of 4.1% due to its proportionality of LY. The ratio of LY values under excitation with alpha- and gamma-rays (alpha/gamma ratio) was also determined. The fast component decay time with relative intensity of 146 ns (66%), 142 ns (76%) and 112 ns (76%) was measured in the scintillation decay of Gd3Al2.7Ga2.3O12:Ce, Gd3Al2.4Ga2.6O12:Ce and Gd3Al2Ga3O12:Ce, respectively. Good coincidence time resolution of Gd3Al2Ga3O12:Ce is due to a high initial photon emission rate.
引用
收藏
页码:23 / 29
页数:7
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