Optical nonlinearity of Cu:SrTiO3 composite fabricated by negative ion implantation

被引:9
作者
Takeda, Y.
Plaksin, O. A.
Lu, J.
Kono, K.
Kishimoto, N.
机构
[1] Natl Inst Mat Sci, Nanomat Lab, Tsukuba, Ibaraki 3050003, Japan
[2] SSC RF, IPPE, Obninsk, Russia
关键词
ion implantation; metal nanoparticle; surface plasmon resonancel; nonlinear dielectric constant; pump-probe method; dispersion;
D O I
10.1016/j.nimb.2006.04.140
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
Optical nonlinearity and dispersion were studied for Cu nanoparticle composite. Negative Cu- ions with 60 keV were applied for implanting into SrTiO3 at a flux of 10 mu A/cm(2) up to a total fluence of 1 x 10(17) ions/cm(2). The steady-state optical spectrum of Cu-implanted SrTiO3 showed a surface plasmon resonance resulting from the formation of nanoparticles. Transient transmission and reflection were measured by the pump-probe method with a femtosecond laser system. Optical nonlinearity originated from Cu:SrTiO3 nanoparticle composite and from SrTiO3 matrix overlap, in measured transient spectra. The nonlinear component of Cu:SrTiO3 composite was extracted from the transient spectra with the difference of time response. Nonlinear dielectric coefficient and dispersion around the surface plasmon resonance were derived from extracted transient spectra. The dispersion was compared with a local electric field factor. (c) 2006 Elsevier B.V. All rights reserved.
引用
收藏
页码:372 / 376
页数:5
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