NOx Storage-Reduction with CO over Combined Catalysts

被引:1
作者
Xiao, Jianhua [1 ]
Li, Xuehui [2 ]
Wang, Lefu [2 ]
机构
[1] Guangdong Police Coll, PRD Publ Safety Inst, Guangzhou 510230, Guangdong, Peoples R China
[2] South China Univ Technol, Sch Chem & Energy Engn, Guangzhou, Guangdong 510640, Peoples R China
来源
ADVANCES IN ENVIRONMENTAL TECHNOLOGIES, PTS 1-6 | 2013年 / 726-731卷
基金
中国国家自然科学基金;
关键词
NO oxidation-storage; NOx storage-reduction; Pt/Ba/Al2O3; Mn/Ba/Al2O3; combined catalyst; OXIDATION; MECHANISMS; FTIR;
D O I
10.4028/www.scientific.net/AMR.726-731.2214
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The combined catalysts Mn/Ba/Al2O3-Pt/Ba/Al2O3 and Mn/Ba/Al2O3+Pt/Ba/Al2O3 for NOx storage-reduction were investigated. Mn/Ba/Al2O3 indicated high activity of NO oxidation and NOx storage in the oxidation-storage reaction and certain reduction activity in the storage-reduction reaction. The combination of Pt/Ba/Al2O3 with Mn/Ba/Al2O3 could enhance the activity of NOx storage-reduction under dynamic lean-rich burn conditions. Compared to Pt/Ba/Al2O3 catalyst, although the Pt content decreased half over Mn/Ba/Al2O3-Pt/Ba/Al2O3 and Mn/Ba/Al2O3+Pt/Ba/Al2O3, the NOx conversion increased 9.4% and 6.3% at 350 degrees C. The pollutions such as NOx and CO could be eliminated effectively over two combined catalysts with low Pt content under dynamic lean-rich burn conditions.
引用
收藏
页码:2214 / +
页数:3
相关论文
共 50 条
[41]   The influence of Pt loading and dispersion on the NOx storage and reduction performance of Pt/K2CO3/Co1Mg2Al1Ox catalysts [J].
Zhang, Cheng ;
Yan, Qinghua ;
Gui, Rongrong ;
Chen, Sining ;
Gao, Yanshan ;
Yu, Feng ;
Wang, Qiang .
CATALYSIS TODAY, 2020, 339 :148-158
[42]   FTIR analysis of storage behavior and sulfur tolerance in barium-based NOx storage and reduction (NSR) catalysts [J].
Fanson, PT ;
Horton, MR ;
Delgass, WN ;
Lauterbach, J .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2003, 46 (02) :393-413
[43]   Support Effects and Chemical Gradients along the Catalyst Bed in NOx Storage-Reduction Studied by Space- and Time-Resolved In Situ DRIFTS [J].
Maeda, Nobutaka ;
Urakawa, Atsushi ;
Baiker, Alfons .
JOURNAL OF PHYSICAL CHEMISTRY C, 2009, 113 (38) :16724-16735
[44]   NOx storage and reduction over potassium titanate nanobelt-based catalyst with high storage capacity [J].
Shen, Weihua ;
Nitta, Atsue ;
Chen, Zhi ;
Eda, Tomonori ;
Yoshida, Akihiro ;
Naito, Shuichi .
JOURNAL OF CATALYSIS, 2011, 280 (02) :161-167
[45]   Unique Compensation Effects of Heavy Metals and Phosphorus Copoisoning over NOx Reduction Catalysts [J].
Zhang, Pan ;
Wang, Penglu ;
Impeng, Sarawoot ;
Lan, Tianwei ;
Liu, Xiangyu ;
Zhang, Dengsong .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2022, 56 (17) :12553-12562
[46]   Pt dispersion effects during NOx storage and reduction on Pt/BaO/Al2O3 catalysts [J].
Clayton, Robert D. ;
Harold, Michael P. ;
Balakotaiah, Vemuri ;
Wan, C. Z. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2009, 90 (3-4) :662-676
[47]   Selective Catalytic Reduction of NOx by CO over Doubly Promoted MeMo/Nb2O5 Catalysts (Me = Pt, Ni, or Co) [J].
Nascimento, Joao Pedro S. ;
Oton, Lais E. ;
Oliveira, Alcineia C. ;
Rodriguez-Aguado, Elena ;
Rodriguez-Castellon, Enrique ;
Araujo, Rinaldo S. ;
Souza, Monique S. ;
Lang, Rossano .
CATALYSTS, 2020, 10 (09) :1-22
[48]   Reaction Kinetics of Aged NOx Storage Catalysts [J].
Hauff, Karin ;
Tuttlies, Ute ;
Eigenberger, Gerhart ;
Nieken, Ulrich .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2013, 52 (25) :8399-8409
[49]   Non-thermal plasma assisted NOx storage and reduction over a cobalt-containing Pd catalyst using H2 and/or CO as reductants [J].
Zhang, Zhao-shun ;
Crocker, Mark ;
Yu, Li-mei ;
Wang, Xin-kui ;
Bai, Zhi-feng ;
Shi, Chuan .
CATALYSIS TODAY, 2015, 258 :175-182
[50]   Role of the Mg/Al atomic ratio in hydrotalcite-based catalysts for NOx storage/reduction [J].
Fornasari, G ;
Glöckler, R ;
Livi, M ;
Vaccari, A .
APPLIED CLAY SCIENCE, 2005, 29 (3-4) :258-266