Polydopamine tethered enzyme/metal-organic framework composites with high stability and reusability

被引：188

作者：

Wu, Xiaoling ^{[1
]}

Yang, Cheng ^{[1
]}

Ge, Jun ^{[1
]}

Liu, Zheng ^{[1
]}

机构：

[1] Tsinghua Univ, Dept Chem Engn, Key Lab Ind Biocatalysis, Minist Educ, Beijing 100084, Peoples R China

来源：

NANOSCALE | 2015年 / 7卷 / 45期

基金：

中国国家自然科学基金; 北京市自然科学基金;

关键词：

IMPARTING FUNCTIONALITY; ENZYMES;

D O I：

10.1039/c5nr05190h

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

An enzyme/metal-organic framework (MOF) composite with both highly stable and easily reusable features was prepared via tethering enzyme/MOF nanocrystals with polydopamine (PDA). The micrometer-sized PDA tethered enzyme/MOF composite can be easily repeatedly used without obvious activity loss, promising for efficient enzymatic catalysis at low cost with long-term operational stability under harsh conditions.

引用

收藏

页码：18883 / 18886

页数：4

相关论文

共 19 条

[1] How Can Proteins Enter the Interior of a MOF? Investigation of Cytochrome c Translocation into a MOF Consisting of Mesoporous Cages with Microporous Windows [J].

Chen, Yao ;

Lykourinou, Vasiliki ;

Vetromile, Carissa ;

Tran Hoang ;

Ming, Li-June ;

Larsen, Randy W. ;

Ma, Shengqian .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (32) :13188-13191

[2] The Chemistry and Applications of Metal-Organic Frameworks [J].

Furukawa, Hiroyasu ;

Cordova, Kyle E. ;

O'Keeffe, Michael ;

Yaghi, Omar M. .

SCIENCE, 2013, 341 (6149) :974-+

[3] Bio-functionalization of metal-organic frameworks by covalent protein conjugation [J].

Jung, Suhyun ;

Kim, Youngmee ;

Kim, Sung-Jin ;

Kwon, Tae-Hwan ;

Huh, Seong ;

Park, Seongsoon .

CHEMICAL COMMUNICATIONS, 2011, 47 (10) :2904-2906

[4] Mussel-inspired surface chemistry for multifunctional coatings [J].

Lee, Haeshin ;

Dellatore, Shara M. ;

Miller, William M. ;

Messersmith, Phillip B. .

SCIENCE, 2007, 318 (5849) :426-430

[5] Single-molecule mechanics of mussel adhesion [J].

Lee, Haeshin ;

Scherer, Norbert F. ;

Messersmith, Phillip B. .

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2006, 103 (35) :12999-13003

[6] Biomimetic mineralization of metal-organic frameworks as protective coatings for biomacromolecules [J].

Liang, Kang ;

Ricco, Raffaele ;

Doherty, Cara M. ;

Styles, Mark J. ;

Bell, Stephen ;

Kirby, Nigel ;

Mudie, Stephen ;

Haylock, David ;

Hill, Anita J. ;

Doonan, Christian J. ;

Falcaro, Paolo .

NATURE COMMUNICATIONS, 2015, 6

[7] Multiple-Interaction Ligands Inspired by Mussel Adhesive Protein: Synthesis of Highly Stable and Biocompatible Nanoparticles [J].

Ling, Daishun ;

Park, Wooram ;

Park, Yong Il ;

Lee, Nohyun ;

Li, Fangyuan ;

Song, Changyeong ;

Yang, Su-Geun ;

Choi, Seung Hong ;

Na, Kun ;

Hyeon, Taeghwan .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2011, 50 (48) :11360-11365

[8] Imparting functionality to a metal-organic framework material by controlled nanoparticle encapsulation [J].

Lu, Guang ;

Li, Shaozhou ;

Guo, Zhen ;

Farha, Omar K. ;

Hauser, Brad G. ;

Qi, Xiaoying ;

Wang, Yi ;

Wang, Xin ;

Han, Sanyang ;

Liu, Xiaogang ;

DuChene, Joseph S. ;

Zhang, Hua ;

Zhang, Qichun ;

Chen, Xiaodong ;

Ma, Jan ;

Loo, Say Chye Joachim ;

Wei, Wei D. ;

Yang, Yanhui ;

Hupp, Joseph T. ;

Huo, Fengwei .

NATURE CHEMISTRY, 2012, 4 (04) :310-316

[9] Immobilization of MP-11 into a Mesoporous Metal-Organic Framework, MP-11@mesoMOF: A New Platform for Enzymatic Catalysis [J].

Lykourinou, Vasiliki ;

Chen, Yao ;

Wang, Xi-Sen ;

Meng, Le ;

Tran Hoang ;

Ming, Li-June ;

Musselman, Ronald L. ;

Ma, Shengqian .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (27) :10382-10385

[10] One-Pot Synthesis of Protein-Embedded Metal-Organic Frameworks with Enhanced Biological Activities [J].

Lyu, Fengjiao ;

Zhang, Yifei ;

Zare, Richard N. ;

Ge, Jun ;

Liu, Zheng .

NANO LETTERS, 2014, 14 (10) :5761-5765