Preparation and Photocatalytic Properties of Sr2-xBaxTa3O10-yNz Nanosheets

被引：24
|
作者：
Ida, Shintaro [1 ,2 ,3 ]
Okamoto, Yohei [1 ]
Hagiwara, Hidehisa [1 ,2 ]
Ishihara, Tatsumi [1 ,2 ]
机构：
[1] Kyushu Univ, Dept Appl Chem, Fac Engn, Nishi Ku, Fukuoka 8190395, Japan
[2] Kyushu Univ, Int Inst Carbon Neutral Energy Res I2CNER, Nishi Ku, Fukuoka 8190395, Japan
[3] Japan Sci & Technol Agcy, Precursory Res Embryon Sci & Technol PRESTO, Kawaguchi, Saitama 3320012, Japan
来源：
CATALYSTS | 2013年 / 3卷 / 01期
关键词：
nanosheet; water splitting; exfoliation; LAYERED PEROVSKITE; HYDROGEN-PRODUCTION; NIOBATE NANOSHEETS; OXIDE NANOSHEETS; CHEMICAL PROCESS; CALCIUM NIOBATE; EXFOLIATION; WATER; FILMS;
D O I：
10.3390/catal3010001
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Sr2-xBaxTa3O10-yNz (x = 0.0, 0.5, 1.0) nanosheets were prepared by exfoliating layered perovskite compounds (CsSr2-xBaxTa3O10-yNz). The Sr1.5Ba0.5Ta3O9.7N0.2 nanosheet showed the highest photocatalytic activity for H-2 production from the water/methanol system among the Sr2-xBaxTa3O9.7N0.2 nanosheets prepared. In addition, Rh-loaded Sr1.5Ba0.5Ta3O9.6N0.3 nanosheet showed the photocatalytic activity for oxygen and hydrogen production from water. The ratio of hydrogen to oxygen evolved was around two. These results indicate that the Rh-loaded Sr1.5Ba0.5Ta3O9.6N0.3 nanosheet is a potential catalyst for photocatalytic water splitting.
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页码：1 / 10
页数：10
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