Ternary photocatalyst of atomic-scale Pt coupled with MoS2 co-loaded on TiO2 surface for highly efficient degradation of gaseous toluene

被引:58
作者
Qu, Jiafu [1 ]
Chen, Dongyun [1 ]
Li, Najun [1 ]
Xu, Qingfeng [1 ]
Li, Hua [1 ]
He, Jinghui [1 ]
Lu, Jianmei [1 ]
机构
[1] Soochow Univ, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
TiO2; nanosheets; Molybdenum disulfide; Atomic-scale Pt; Photocatalytic oxidation; Toluene removal; SINGLE-ATOM; OXIDATION; NANOSHEETS; PHOTODEGRADATION; HETEROJUNCTIONS; NANOCOMPOSITES; NANOPARTICLES; IRRADIATION; ADSORPTION; COCATALYST;
D O I
10.1016/j.apcatb.2019.117877
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Photocatalysis by semiconducting materials loaded with non-metal or noble metals is an excellent strategy for removal of gaseous toluene. Herein, a new photocatalytic system was successfully prepared via simultaneously coupling atomic-scale Pt with MoS2 as co-catalysts to load on the surface of TiO2. The obtained photocatalysts exhibited good performance in toluene degradation by promoting the separation of photogenerated electron-hole pairs. The most efficient toluene degradation was achieved by the photocatalyst with a content of 2.0 wt% Pt-MT-1.0 (i.e., coupling 2.0 wt% atomic-scale Pt with 1.0 wt% MoS2), with a conversion ratio of 91.5%. This conversion ratio was higher than those of platinum-free MT-1.0 (33.9%) and pure TiO2 (72.3%). The results demonstrate the potential application of this new nanocomposite for efficient photocatalytic degradation of toluene.
引用
收藏
页数:8
相关论文
共 50 条
  • [31] TiO2/SnO2 double-shelled hollow spheres-highly efficient photocatalyst for the degradation of rhodamine B
    Yuan, Jujun
    Zhang, Xianke
    Li, Hongdong
    Wang, Kai
    Gao, Shiyong
    Yin, Zhen
    Yu, Huajun
    Zhu, Xiurong
    Xiong, Zuzhou
    Xie, Yingmao
    CATALYSIS COMMUNICATIONS, 2015, 60 : 129 - 133
  • [32] Dual active sites fabricated through atomic layer deposition of TiO2 on MoS2 nanosheet arrays for highly efficient electroreduction of CO2 to ethanol
    Qi, Feixuanyu
    Liu, Kang
    Ma, De-Kun
    Cai, Fangfang
    Liu, Min
    Xu, Quanlong
    Chen, Wei
    Qi, Chenze
    Yang, Dongpeng
    Huang, Shaoming
    JOURNAL OF MATERIALS CHEMISTRY A, 2021, 9 (11) : 6790 - 6796
  • [33] Binary composite MoS2/TiO2 nanotube arrays as a recyclable and efficient photocatalyst for solar water disinfection
    Yan, Huiling
    Liu, Lizhi
    Wang, Rong
    Zhu, Wenxin
    Ren, Xinyi
    Luo, Linpin
    Zhang, Xu
    Luo, Shijia
    Ai, Xuelian
    Wang, Jianlong
    CHEMICAL ENGINEERING JOURNAL, 2020, 401
  • [34] Ternary hybrid Au@Pt-TiO2 nanocomposites: Highly thermally stable photocatalyst with highly efficient visible-light photocatalytic activity
    Mezni, Amine
    JOURNAL OF MATERIALS RESEARCH AND TECHNOLOGY-JMR&T, 2020, 9 (06): : 15263 - 15272
  • [35] Potassium Poly(heptazine imide) Coupled with Ti3C2 MXene-Derived TiO2 as a Composite Photocatalyst for Efficient Pollutant Degradation
    Chen, Binbin
    Lu, Weiwei
    Xu, Peng
    Yao, Kaisheng
    ACS OMEGA, 2023, 8 (12): : 11397 - 11405
  • [36] Photocatalytic degradation of gaseous toluene over Ag-doping TiO2 nanotube powder prepared by anodization coupled with impregnation method
    Li, Xinyong
    Zou, Xuejun
    Qu, Zhenping
    Zhao, Qidong
    Wang, Lianzhou
    CHEMOSPHERE, 2011, 83 (05) : 674 - 679
  • [37] Tailored highly efficient Co-doped TiO2/CoTiO3 heterojunction photocatalyst for methylene blue degradation under visible light
    Basumatary, Rajmoni
    Basumatary, Bablu
    Konwar, Dimpul
    Ramchiary, Anjalu
    JOURNAL OF THE KOREAN CERAMIC SOCIETY, 2023, 60 (03) : 547 - 559
  • [38] Ameliorative photocatalytic dye degradation performance of ternary Co3O4/MoS2/TiO2 nanocomposite under visible light illumination
    Elavarasan, N.
    Venkatesh, Gopal
    Periyasami, Govindasami
    Sembiring, Kiky Corneliasari
    Lee, Jintae
    Palanisamy, Govindasamy
    JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS, 2025, 171
  • [39] Integrated ternary nanocomposite of TiO2/NiO/reduced graphene oxide as a visible light photocatalyst for efficient degradation of o-chlorophenol
    Sharma, Ajit
    Lee, Byeong-Kyu
    JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2016, 181 : 563 - 573
  • [40] A novel ternary MoS2/MoO3/TiO2 composite for fast photocatalytic degradation of rhodamine B under visible-light irradiation
    Li, Zhenyu
    Cao, Fa
    Wang, Lei
    Chen, Zhiwu
    Ji, Xiaohong
    NEW JOURNAL OF CHEMISTRY, 2020, 44 (02) : 537 - 542