共 50 条
Ternary photocatalyst of atomic-scale Pt coupled with MoS2 co-loaded on TiO2 surface for highly efficient degradation of gaseous toluene
被引:58
|作者:
Qu, Jiafu
[1
]
Chen, Dongyun
[1
]
Li, Najun
[1
]
Xu, Qingfeng
[1
]
Li, Hua
[1
]
He, Jinghui
[1
]
Lu, Jianmei
[1
]
机构:
[1] Soochow Univ, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Peoples R China
基金:
国家重点研发计划;
中国国家自然科学基金;
关键词:
TiO2;
nanosheets;
Molybdenum disulfide;
Atomic-scale Pt;
Photocatalytic oxidation;
Toluene removal;
SINGLE-ATOM;
OXIDATION;
NANOSHEETS;
PHOTODEGRADATION;
HETEROJUNCTIONS;
NANOCOMPOSITES;
NANOPARTICLES;
IRRADIATION;
ADSORPTION;
COCATALYST;
D O I:
10.1016/j.apcatb.2019.117877
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Photocatalysis by semiconducting materials loaded with non-metal or noble metals is an excellent strategy for removal of gaseous toluene. Herein, a new photocatalytic system was successfully prepared via simultaneously coupling atomic-scale Pt with MoS2 as co-catalysts to load on the surface of TiO2. The obtained photocatalysts exhibited good performance in toluene degradation by promoting the separation of photogenerated electron-hole pairs. The most efficient toluene degradation was achieved by the photocatalyst with a content of 2.0 wt% Pt-MT-1.0 (i.e., coupling 2.0 wt% atomic-scale Pt with 1.0 wt% MoS2), with a conversion ratio of 91.5%. This conversion ratio was higher than those of platinum-free MT-1.0 (33.9%) and pure TiO2 (72.3%). The results demonstrate the potential application of this new nanocomposite for efficient photocatalytic degradation of toluene.
引用
收藏
页数:8
相关论文