Signatures of the spin-phonon coupling in Fe1+yTe1-xSex alloys

被引:15
作者
Popovic, Z. V. [1 ]
Lazarevic, N. [1 ]
Bogdanovic, S. [1 ]
Radonjic, M. M. [2 ]
Tanaskovic, D. [2 ]
Hu, Rongwei [3 ]
Lei, Hechang [3 ]
Petrovic, C. [3 ]
机构
[1] Univ Belgrade, Inst Phys Belgrade, Ctr Solid State Phys & New Mat, Belgrade 11080, Serbia
[2] Univ Belgrade, Inst Phys Belgrade, Comp Sci Lab, Belgrade 11080, Serbia
[3] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA
关键词
Magnetically ordered materials; Crystal structure and symmetry; Phonos; Inelastic light scattering; 1ST-PRINCIPLES CALCULATIONS; SUPERCONDUCTIVITY;
D O I
10.1016/j.ssc.2014.05.025
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Raman scattering spectra of Fe1+yTe1-xSex (x=0, y=0.07; x=0.1, y=0.05 and x=0.4, y=0.02) alloys are measured in a temperature range between 20 K and 300 K. The A(1g) and B-1g Raman active modes have been experimentally observed at energies 156 and 198 cm(-1), which is in rather good agreement with the lattice dynamics calculation. The antiferromagnetic spin ordering below 70 K in Fe1.07Te leaves a fingerprint only in the B-1g phonon mode linewidth and energy, whose temperature dependence follows the normalized magnetic susceptibility, indicating the presence of the spin-phonon coupling. The frequency and the linewidth of the A(1g) mode assume a conventional anharmonic temperature dependence in all measured samples, which is also the case for the B-1g mode in the Se doped samples. The linewidth (energy) of the A(1g) mode decreases (increases) with doping, whereas the opposite is seen for the B-1g mode. (C) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码:51 / 55
页数:5
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