Air-based photoelectrochemical cell capturing water molecules from ambient air for hydrogen production

被引:46
作者
Ronge, J. [1 ]
Deng, S. [2 ]
Sree, S. Pulinthanathu [1 ]
Bosserez, T. [1 ]
Verbruggen, S. W. [1 ]
Singh, N. Kumar [1 ]
Dendooven, J. [2 ]
Roeffaers, M. B. J. [1 ]
Taulelle, F. [1 ,3 ]
De Volder, M. [4 ]
Detavernier, C. [2 ]
Martens, J. A. [1 ]
机构
[1] Katholieke Univ Leuven, Ctr Surface Chem & Catalysis, B-3001 Leuven, Belgium
[2] UGent, Dept Solid State Sci, B-9000 Ghent, Belgium
[3] Univ Versailles, Inst Lavoisier, Tectospin, F-78035 Versailles, France
[4] Katholieke Univ Leuven, Dept Mech Engn, B-3001 Leuven, Belgium
基金
欧洲研究理事会;
关键词
ATOMIC LAYER DEPOSITION; MEMBRANE FUEL-CELLS; PHOTOCATALYTIC DECOMPOSITION; CARBON NANOTUBES; TIO2; CATALYST; NANOSTRUCTURES; NANOPARTICLES; INTERFACE; DEVICES;
D O I
10.1039/c4ra05371k
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A system is demonstrated that autonomously produces hydrogen gas using sunlight and outside air as the only inputs. Oxygen and hydrogen formation reactions occur on either side of a monolithic "solar membrane" inserted in a two-compartment photoelectrochemical cell. A surface film of Nafion (R) serves as a solid electrolyte. This proof of concept invites further development of air-based cells.
引用
收藏
页码:29286 / 29290
页数:5
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