Air-based photoelectrochemical cell capturing water molecules from ambient air for hydrogen production

被引:46
作者
Ronge, J. [1 ]
Deng, S. [2 ]
Sree, S. Pulinthanathu [1 ]
Bosserez, T. [1 ]
Verbruggen, S. W. [1 ]
Singh, N. Kumar [1 ]
Dendooven, J. [2 ]
Roeffaers, M. B. J. [1 ]
Taulelle, F. [1 ,3 ]
De Volder, M. [4 ]
Detavernier, C. [2 ]
Martens, J. A. [1 ]
机构
[1] Katholieke Univ Leuven, Ctr Surface Chem & Catalysis, B-3001 Leuven, Belgium
[2] UGent, Dept Solid State Sci, B-9000 Ghent, Belgium
[3] Univ Versailles, Inst Lavoisier, Tectospin, F-78035 Versailles, France
[4] Katholieke Univ Leuven, Dept Mech Engn, B-3001 Leuven, Belgium
基金
欧洲研究理事会;
关键词
ATOMIC LAYER DEPOSITION; MEMBRANE FUEL-CELLS; PHOTOCATALYTIC DECOMPOSITION; CARBON NANOTUBES; TIO2; CATALYST; NANOSTRUCTURES; NANOPARTICLES; INTERFACE; DEVICES;
D O I
10.1039/c4ra05371k
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A system is demonstrated that autonomously produces hydrogen gas using sunlight and outside air as the only inputs. Oxygen and hydrogen formation reactions occur on either side of a monolithic "solar membrane" inserted in a two-compartment photoelectrochemical cell. A surface film of Nafion (R) serves as a solid electrolyte. This proof of concept invites further development of air-based cells.
引用
收藏
页码:29286 / 29290
页数:5
相关论文
共 49 条
  • [1] Efficient solar water splitting by enhanced charge separation in a bismuth vanadate-silicon tandem photoelectrode
    Abdi, Fatwa F.
    Han, Lihao
    Smets, Arno H. M.
    Zeman, Miro
    Dam, Bernard
    van de Krol, Roel
    [J]. NATURE COMMUNICATIONS, 2013, 4
  • [2] Catalytic effect of metal oxides on the oxidation resistance in carbon nanotube-inorganic hybrids
    Aksel, S.
    Eder, D.
    [J]. JOURNAL OF MATERIALS CHEMISTRY, 2010, 20 (41) : 9149 - 9154
  • [3] Synthesis of solar fuels by a novel photoelectrocatalytic approach
    Ampelli, Claudio
    Centi, Gabriele
    Passalacqua, Rosalba
    Perathoner, Siglinda
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2010, 3 (03) : 292 - 301
  • [4] Brillet J, 2012, NAT PHOTONICS, V6, P823, DOI [10.1038/nphoton.2012.265, 10.1038/NPHOTON.2012.265]
  • [5] Shining a Light on Solar Water Splitting
    Chandross, Edwin A.
    [J]. SCIENCE, 2014, 344 (6183) : 469 - 469
  • [6] Interface engineering in nanocarbon-Ta2O5 hybrid photocatalysts
    Cherevan, Alexey S.
    Gebhardt, Paul
    Shearer, Cameron J.
    Matsukawa, Michinori
    Domen, Kazunari
    Eder, Dominik
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2014, 7 (02) : 791 - 796
  • [7] Low-Temperature Atomic Layer Deposition of Platinum Using (Methylcyclopentadienyl)trimethylplatinum and Ozone
    Dendooven, Jolien
    Ramachandran, Ranjith K.
    Devloo-Casier, Kilian
    Rampelberg, Geert
    Filez, Matthias
    Poelman, Hilde
    Marin, Guy B.
    Fonda, Emiliano
    Detavernier, Christophe
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2013, 117 (40) : 20557 - 20561
  • [8] Atomic layer deposition-based synthesis of photoactive TiO2 nanoparticle chains by using carbon nanotubes as sacrificial templates
    Deng, Shaoren
    Verbruggen, Sammy W.
    He, Zhanbing
    Cott, Daire J.
    Vereecken, Philippe M.
    Martens, Johan A.
    Bals, Sara
    Lenaerts, Silvia
    Detavernier, Christophe
    [J]. RSC ADVANCES, 2014, 4 (23) : 11648 - 11653
  • [9] Gas phase photocatalytic water splitting with Rh2-yCryO3/GaN:ZnO in μ-reactors
    Dionigi, Fabio
    Vesborg, Peter C. K.
    Pedersen, Thomas
    Hansen, Ole
    Dahl, Soren
    Xiong, Anke
    Maeda, Kazuhiko
    Domen, Kazunari
    Chorkendorff, Ib
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2011, 4 (08) : 2937 - 2942
  • [10] Domen K., 1980, J CHEM SOC F1, V1, P543