Enhancement of energy storage density in antiferroelectric PbZrO3 films via the incorporation of gold nanoparticles

被引：26
作者：
Li, Yi Zhuo [1 ,2 ]
Wang, Zhan Jie [1 ,2 ,3 ]
Bai, Yu [1 ]
Liu, Wei [1 ,2 ]
Zhang, Zhi Dong [1 ,2 ]
机构：
[1] Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang, Liaoning, Peoples R China
[2] Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang, Liaoning, Peoples R China
[3] Shenyang Univ Technol, Sch Mat Sci & Engn, Shenyang, Liaoning, Peoples R China
来源：
JOURNAL OF THE AMERICAN CERAMIC SOCIETY | 2019年 / 102卷 / 09期
关键词：
energy storage; lead zirconate; nanocomposites; nanoparticles; GRAIN-SIZE; ELECTRICAL-PROPERTIES; THIN-FILM; PERFORMANCE; CERAMICS; MICROSTRUCTURE; POLARIZATION; FIELD;
D O I：
10.1111/jace.16408
中图分类号：
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号：
0805 ; 080502 ;
摘要：
In this work, antiferroelectric Au-PbZrO3 (Au-PZO) nanocomposite thin films were prepared by chemical solution deposition (CSD), and the effects of Au concentration on the antiferroelectric properties and the recoverable energy density were investigated. The results showed that the optimal Au concentration in the Au-PZO nanocomposite thin films was about 1mol% for structural and electric properties. In the Au-PZO nanocomposite thin films with 1mol% Au, Au nanoparticles (NPs) were distributed uniformly in the perovskite PZO matrix. Moreover, the recoverable energy density was 10.8J/cm(3) at 600kV/cm, which is 42% higher than that of the pure PZO films. The results demonstrate that adding an appropriate amount of noble metal NPs in antiferroelectric thin films is an effective method to improve the energy storage properties.
引用
收藏
页码：5253 / 5261
页数：9
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