Atmospheric wet deposition of nitrogen in a subtropical watershed in China: characteristics of and impacts on surface water quality

被引:35
作者
Hao, Zhuo [1 ]
Gao, Yang [1 ,2 ]
Yang, Tiantian [3 ]
Tian, Jing [1 ,2 ]
机构
[1] Chinese Acad Sci, Key Lab Ecosyst Network Observat & Modeling, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Univ Calif Irvine, Dept Civil & Environm Engn, Irvine, CA 92697 USA
关键词
N wet deposition; Watershed; Rainfall-runoff; Baseflow; Water quality; POLYCYCLIC AROMATIC-HYDROCARBONS; SEDIMENT LOAD; RUNOFF; TERRESTRIAL; PHOSPHORUS; LOSSES; SOUTHEAST; AREA; BAY; DRY;
D O I
10.1007/s11356-017-8532-5
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Atmospheric wet deposition of nitrogen (N) is an important process in global N cycling, having significant impacts on both water quality and aquatic ecosystems worldwide. The aims of this study were to clarify the N wet deposition first flush effect and estimate the contribution of N wet deposition on both N export and water quality in a subtropical watershed. Results showed that total nitrogen (TN) flux was 41.72 kg N hm(-2) year(-1) and dissolved total nitrogen (DTN) was 23.18 kg N hm(-2) year(-1), respectively. Light rain events lead to the highest DTN and dissolve inorganic nitrogen (DIN) concentrations of wet deposition. Rainstorm concentrations were lowest during spring rainfall-runoff events. In contrast to the baseflow, the different N forms were higher than they were under the rainfall-runoff. Rainfall event contributions on N export were greater than 93.2% in the watershed for the whole year. Finally, TN concentrations were higher than river eutrophication thresholds for the entire watershed.
引用
收藏
页码:8489 / 8503
页数:15
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