Picometre-precision analysis of scanning transmission electron microscopy images of platinum nanocatalysts

被引:211
作者
Yankovich, Andrew B. [1 ]
Berkels, Benjamin [2 ,3 ]
Dahmen, W. [2 ,4 ]
Binev, P. [2 ]
Sanchez, S. I. [5 ]
Bradley, S. A. [5 ]
Li, Ao [1 ]
Szlufarska, Izabela [1 ]
Voyles, Paul M. [1 ]
机构
[1] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA
[2] Univ S Carolina, Interdisciplinary Math Inst, Columbia, SC 29208 USA
[3] Rhein Westfal TH Aachen, Aachen Inst Adv Study Computat Engn Sci AICES, D-52062 Aachen, Germany
[4] Rhein Westfal TH Aachen, Inst Geometr & Prakt Math, D-52056 Aachen, Germany
[5] UOP LLC Honeywell Co, Des Plaines, IA 60017 USA
基金
美国国家科学基金会;
关键词
THERMAL VIBRATIONS; CATALYTIC-ACTIVITY; NANOPARTICLES; CONTRACTION;
D O I
10.1038/ncomms5155
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Measuring picometre-scale shifts in the positions of individual atoms in materials provides new insight into the structure of surfaces, defects and interfaces that influence a broad variety of materials' behaviour. Here we demonstrate sub-picometre precision measurements of atom positions in aberration-corrected Z-contrast scanning transmission electron microscopy images based on the non-rigid registration and averaging of an image series. Non-rigid registration achieves five to seven times better precision than previous methods. Non-rigidly registered images of a silica-supported platinum nanocatalyst show pm-scale contraction of atoms at a (111)/(111) corner towards the particle centre and expansion of a flat (111) facet. Sub-picometre precision and standardless atom counting with <1 atom uncertainty in the same scanning transmission electron microscopy image provide new insight into the three-dimensional atomic structure of catalyst nanoparticle surfaces, which contain the active sites controlling catalytic reactions.
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页数:7
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