Nonequilibrium magnetic properties in oxygen-rich LaMnO3 nanoparticles

被引:3
作者
Xue, Kaiyuan [1 ]
He, Feifei [1 ]
Zhang, Jiang [1 ]
Tang, Lingyun [1 ]
Chen, Xi [1 ]
Mao, Zhongquan [1 ]
机构
[1] South China Univ Technol, Sch Phys & Optoelect, Guangzhou, Guangdong, Peoples R China
关键词
nonequilibrium property; spin glass; irreversible phenomenon; magnetic nanoparticle; BEHAVIOR; PHASE; STATE;
D O I
10.1088/1361-648X/ab22e9
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Nonequilibrium magnetic properties of oxygen-rich LaMnO3.21 nanoparticles have been investigated by comprehensive magnetic measurements. The composition falls in the metamagnetic canted spin region of the magnetic phase diagram. However, the zero-fieldcooling memory effect and frequency-dependent AC susceptibility reveal a re-entrant glassy state at low temperature. In contrast to the super-spin glass or cluster glass that re-enter from the high-temperature ferromagnetic state in previous studies, analyses based on the power law and Vogel-Fulcher law indicate strongly a conventional spin glass nature. As the magnetic field increases, an anomalous enhancement of the irreversible temperature is observed, suggesting a field-induced nonequilibrium magnetic state. These results can be understood by considering the interaction between the antiferromagnetic clusters and the metamagnetic canted-spin matrix inside the nanoparticles.
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页数:6
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