Cooperative strings in glassy nanoparticles

被引:16
作者
Arutkin, Maxence [1 ]
Raphael, Elie [1 ]
Forrest, James A. [1 ,2 ,3 ,4 ]
Salez, Thomas [1 ,2 ,5 ]
机构
[1] PSL Res Univ, ESPCI ParisTech, UMR CNRS Gulliver 7083, Lab Physicochim Theor, F-75005 Paris, France
[2] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada
[3] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada
[4] Univ Waterloo, Guelph Waterloo Phys Inst, Waterloo, ON N2L 3G1, Canada
[5] Hokkaido Univ, Global Stn Soft Matter, Global Inst Collaborat Res & Educ, Sapporo, Hokkaido 0600808, Japan
关键词
THIN POLYMER-FILMS; TRANSITION TEMPERATURE; FORMING LIQUIDS; JAMMING TRANSITION; HARD CONFINEMENT; FREE SURFACES; DYNAMICS; RELAXATION; DEPENDENCE; NANOSPHERES;
D O I
10.1039/c6sm00724d
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Motivated by recent experimental results on glassy polymer nanoparticles, we develop a minimal theoretical framework for the glass transition in spherical confinement. This is accomplished using our cooperative-string model for supercooled dynamics, that was successful at recovering the bulk phenomenology and describing the thin-film anomalies. In particular, we obtain predictions for the mobile-layer thickness as a function of temperature, and for the effective glass-transition temperature as a function of the radius of the spherical nanoparticle - including the existence of a critical particle radius below which vitrification never occurs. Finally, we compare the theoretical results to experimental data on polystyrene from the recent literature, and we discuss the latter.
引用
收藏
页码:141 / 146
页数:6
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