Hybrid inorganic-organic tandem solar cells for broad absorption of the solar spectrum

被引：19

作者：

Speirs, M. J. ^{[1
]}

Groeneveld, B. G. H. M. ^{[1
]}

Protesescu, L. ^{[2
,3
]}

Piliego, C. ^{[1
]}

Kovalenko, M. V. ^{[2
,3
]}

Loi, M. A. ^{[1
]}

机构：

[1] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands

[2] ETH, Dept Chem & Appl Biosci, CH-8093 Zurich, Switzerland

[3] EMPA Swiss Fed Labs Mat Sci & Technol, CH-8600 Dubendorf, Switzerland

来源：

PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 2014年 / 16卷 / 17期

关键词：

EFFICIENCY; PBS; PHOTOCURRENT; FILMS;

D O I：

10.1039/c4cp00846d

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We report the first hybrid tandem solar cell with solution processable active layers using colloidal PbS quantum dots (QDs) as the front subcell in combination with a polymer-fullerene rear subcell. Al/WO3 is introduced as an interlayer, yielding an open circuit voltage (V-OC) equal to about 92% of the sum of the V-OC of the subcells. The device exhibits a power conversion efficiency of 1.8%. Optical simulations of various tandem configurations show that combining PbS QDs with small-bandgap polymers is a promising strategy to obtain tandem solar cells with a very broad absorption range and a high short circuit current.

引用

页码：7672 / 7676

页数：5

共 30 条

[1] Highly efficient organic tandem solar cells: a follow up review [J].

Ameri, Tayebeh ;

Li, Ning ;

Brabec, Christoph J. .

ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (08) :2390-2413

[2] Fabrication, Optical Modeling, and Color Characterization of Semitransparent Bulk-Heterojunction Organic Solar Cells in an Inverted Structure [J].

Ameri, Tayebeh ;

Dennler, Gilles ;

Waldauf, Christoph ;

Azimi, Hamed ;

Seemann, Andrea ;

Forberich, Karen ;

Hauch, Jens ;

Scharber, Markus ;

Hingerl, Kurt ;

Brabec, Christoph J. .

ADVANCED FUNCTIONAL MATERIALS, 2010, 20 (10) :1592-1598

[3] Organic tandem solar cells: A review [J].

Ameri, Tayebeh ;

Dennler, Gilles ;

Lungenschmied, Christoph ;

Brabec, Christoph J. .

ENERGY & ENVIRONMENTAL SCIENCE, 2009, 2 (04) :347-363

[4] Solution-Processed Nanocrystal Quantum Dot Tandem Solar Cells [J].

Choi, Joshua J. ;

Wenger, Whitney N. ;

Hoffman, Rachel S. ;

Lim, Yee-Fun ;

Luria, Justin ;

Jasieniak, Jacek ;

Marohn, John A. ;

Hanrath, Tobias .

ADVANCED MATERIALS, 2011, 23 (28) :3144-+

[5] Design rules for donors in bulk-heterojunction tandem solar cells-towards 15 % energy-conversion efficiency [J].

Dennler, Gilles ;

Scharber, Markus C. ;

Ameri, Tayebeh ;

Denk, Patrick ;

Forberich, Karen ;

Waldauf, Christoph ;

Brabec, Christoph J. .

ADVANCED MATERIALS, 2008, 20 (03) :579-+

[6]

He ZC, 2012, NAT PHOTONICS, V6, P591, DOI [10.1038/nphoton.2012.190, 10.1038/NPHOTON.2012.190]

[7] Inverse relation between photocurrent and absorption layer thickness in polymer solar cells [J].

Hoppe, Harald ;

Shokhovets, Sviatoslav ;

Gobsch, Gerhard .

PHYSICA STATUS SOLIDI-RAPID RESEARCH LETTERS, 2007, 1 (01) :R40-R42

[8] Highly efficient organic tandem solar cells using an improved connecting architecture [J].

Janssen, A. G. F. ;

Riedl, T. ;

Hamwi, S. ;

Johannes, H.-H. ;

Kowalsky, W. .

APPLIED PHYSICS LETTERS, 2007, 91 (07)

[9] Combined optical and electrical modeling of polymer:fullerene bulk heterojunction solar cells [J].

Kotlarski, Jan D. ;

Blom, Paul W. M. ;

Koster, Lambert. J. A. ;

Lenes, Martijn ;

Slooff, Lenneke H. .

JOURNAL OF APPLIED PHYSICS, 2008, 103 (08)

[10] Accurate efficiency determination and stability studies of conjugated polymer/fullerene solar cells [J].

Kroon, JM ;

Wienk, MM ;

Verhees, WJH ;

Hummelen, JC .

THIN SOLID FILMS, 2002, 403 :223-228

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