The non-Markovian master equation for stochastically perturbed systems: Effect on spectral lineshape

被引:0
|
作者
Gangopadhyay, G
Ray, DS
机构
[1] INDIAN ASSOC CULTIVAT SCI, DEPT PHYS CHEM, CALCUTTA 700032, W BENGAL, INDIA
[2] SN BOSE NATL CTR BASIC SCI, CALCUTTA 700064, W BENGAL, INDIA
来源
JOURNAL OF MOLECULAR STRUCTURE-THEOCHEM | 1996年 / 361卷
关键词
D O I
10.1016/0166-1280(95)04301-2
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Based on the system-reservoir model in which the intermediate states of the system are perturbed by stochastic interaction with the surroundings, we have generalized the master equation for the description of quantum dissipative processes and applied it to a three-level system to calculate transient optical response in pump-probe spectroscopy. We have shown that while the two damping processes act independently in the Markovian description, the interference of stochastic and system-reservoir interactions and the resulting non-lorentzian structure of the band-shape function appear as the essential non-Markovian features in the dissipative dynamics.
引用
收藏
页码:49 / 56
页数:8
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