Better thermoelectrics through glass-like crystals

被引：247

作者：

Beekman, Matt ^{[1
]}

Morelli, Donald T. ^{[2
]}

Nolas, George S. ^{[3
]}

机构：

[1] Oregon Inst Technol, Dept Nat Sci, Klamath Falls, OR 97601 USA

[2] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA

[3] Univ S Florida, Dept Phys, Tampa, FL 33620 USA

来源：

NATURE MATERIALS | 2015年 / 14卷 / 12期

关键词：

LATTICE THERMAL-CONDUCTIVITY; FILLED SKUTTERUDITES; PERFORMANCE; FIGURE; MERIT; CONVERGENCE; EFFICIENCY; DESIGN; BANDS;

D O I：

10.1038/nmat4461

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Twenty years ago, the 'phonon-glass, electron-crystal' concept changed thinking in thermoelectric materials research, resulting in new high-performance materials and an increased focus on controlling structure and chemical bonding to minimize irreversible heat transport in crystals. © 2015 Macmillan Publishers Limited. All rights reserved.

引用

页码：1182 / 1185

页数：4

共 45 条

[1]

Altenkirch E, 1909, PHYS Z, V10, P560

[2]

[Anonymous], 2014, PHYS CHEM INORGANIC

[3] PREPARATION AND STRUCTURAL INVESTIGATIONS OF ANTI-MONIDES WITH THE LAFE4P12 STRUCTURE [J].

BRAUN, DJ ;

JEITSCHKO, W .

JOURNAL OF THE LESS-COMMON METALS, 1980, 72 (01) :147-156

[4] Yb14MnSb11:: New high efficiency thermoelectric material for power generation [J].

Brown, SR ;

Kauzlarich, SM ;

Gascoin, F ;

Snyder, GJ .

CHEMISTRY OF MATERIALS, 2006, 18 (07) :1873-1877

[5] LOWER LIMIT TO THE THERMAL-CONDUCTIVITY OF DISORDERED CRYSTALS [J].

CAHILL, DG ;

WATSON, SK ;

POHL, RO .

PHYSICAL REVIEW B, 1992, 46 (10) :6131-6140

[6] Ultralow thermal conductivity in disordered, layered WSe2 crystals [J].

Chiritescu, Catalin ;

Cahill, David G. ;

Nguyen, Ngoc ;

Johnson, David ;

Bodapati, Arun ;

Keblinski, Pawel ;

Zschack, Paul .

SCIENCE, 2007, 315 (5810) :351-353

[7] Avoided crossing of rattler modes in thermoelectric materials [J].

Christensen, Mogens ;

Abrahamsen, Asger B. ;

Christensen, Niels B. ;

Juranyi, Fanni ;

Andersen, Niels H. ;

Lefmann, Kim ;

Andreasson, Jakob ;

Bahl, Christian R. H. ;

Iversen, Bo B. .

NATURE MATERIALS, 2008, 7 (10) :811-815

[8] CsBi4Te6:: A high-performance thermoelectric material for low-temperature applications [J].

Chung, DY ;

Hogan, T ;

Brazis, P ;

Rocci-Lane, M ;

Kannewurf, C ;

Bastea, M ;

Uher, C ;

Kanatzidis, MG .

SCIENCE, 2000, 287 (5455) :1024-1027

[9] Glasslike heat conduction in high-mobility crystalline semiconductors [J].

Cohn, JL ;

Nolas, GS ;

Fessatidis, V ;

Metcalf, TH ;

Slack, GA .

PHYSICAL REVIEW LETTERS, 1999, 82 (04) :779-782

[10]

Dong Y., 2015, CHEMPHYSCHEM

← 1 2 3 4 5 →