One-pot Synthesis of Nitrogen and Phosphorus Co-doped Graphene and Its Use as High-performance Electrocatalyst for Oxygen Reduction Reaction

被引:49
作者
Dong, Liye [1 ]
Hu, Chuangang [1 ]
Huang, Xianke [1 ]
Chen, Nan [1 ]
Qu, Liangti [1 ]
机构
[1] Beijing Inst Technol, Minist Educ China, Beijing Key Lab Photoelect Electrophoton Convers, Sch Chem,Key Lab Cluster Sci, Beijing, Peoples R China
基金
北京市自然科学基金;
关键词
co-doped graphene; nitrogen; one-pot synthesis; oxygen reduction reaction; phosphorus; METAL-FREE ELECTROCATALYSTS; CARBON NANOTUBE ARRAYS; REDUCED GRAPHENE; FUEL-CELLS; CATALYSTS; SULFUR; OXIDE; NANOSHEETS; BORON;
D O I
10.1002/asia.201500707
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this study, N,P co-doped graphene (NPG) was prepared by a one-step pyrolysis using a mixture of graphene oxide and hexachlorocyclotriphosphazene (HCCP), in which HCCP was used as both the N and P source. Furthermore, it is shown that NPG electrodes, as efficient metal-free electrocatalysts, have a high onset potential, high current density, and long-term stability for the oxygen reduction reaction.
引用
收藏
页码:2608 / 2613
页数:6
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