Influence of catalyst packing configuration on the discharge characteristics of dielectric barrier discharge reactors: A numerical investigation

被引:34
作者
Gadkari, Siddharth [1 ,2 ]
Gu, Sai [1 ]
机构
[1] Univ Surrey, Dept Chem & Proc Engn, Guildford GU2 7XH, Surrey, England
[2] Univ Surrey, Ctr Environm & Sustainabil, Guildford GU2 7XH, Surrey, England
基金
英国工程与自然科学研究理事会;
关键词
PLASMA CATALYSIS; ATMOSPHERIC-PRESSURE; DIRECT CONVERSION; GREENHOUSE GASES; METHANE; HYDROCARBONS; REMOVAL; TOLUENE; CO2;
D O I
10.1063/1.5030508
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
A two-dimensional numerical fluid model is developed for studying the influence of packing configurations on dielectric barrier discharge (DBD) characteristics. Discharge current profiles and time averaged electric field strength, electron number density, and electron temperature distributions are compared for the three DBD configurations, plain DBD with no packing, partially packed DBD, and fully packed DBD. The results show that a strong change in discharge behaviour occurs when a DBD is fully packed as compared to partial packing or no packing. While the average electric field strength and electron temperature of a fully packed DBD are higher relative to the other DBD configurations, the average electron density is substantially lower and may impede the DBD reactor performance under certain operating conditions. Possible scenarios of the synergistic effect of the combination of plasma with catalysis are also discussed. (C) 2018 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license.
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收藏
页数:7
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