High spatial resolved cropland coverage and cultivation category determine neonicotinoid distribution in agricultural soil at the provincial scale

被引:26
作者
Chen, Yuanchen [1 ]
Wu, Ruxin [1 ]
Zhang, Li [1 ]
Ling, Jun [1 ]
Yu, Wenfei [1 ]
Shen, Guofeng [2 ]
Du, Wei [3 ,4 ]
Zhao, Meirong [1 ]
机构
[1] Zhejiang Univ Technol, Coll Environm, Res Ctr Environm Sci, Key Lab Microbial Technol Ind Pollut Control Zhej, Hangzhou 310032, Peoples R China
[2] Peking Univ, Coll Urban & Environm Sci, Minist Educ, Lab Earth Surface Proc, Beijing 100871, Peoples R China
[3] Kunming Univ Sci & Technol, Yunnan Prov Key Lab Soil Carbon Sequestrat & Poll, Fac Environm Sci & Engn, Kunming 650500, Yunnan, Peoples R China
[4] East China Normal Univ, Sch Geog Sci, Minist Educ, Key Lab Geog Informat Sci, Shanghai 200241, Peoples R China
基金
中国国家自然科学基金;
关键词
Landuse; Application methods; Spatial distribution; Agricultural soil; Predicting model; ENVIRONMENTAL RISKS; CHINA; CONTAMINATION; INSECTICIDES; RESIDUES; EXPOSURE; PRODUCT; FIELDS; FATE;
D O I
10.1016/j.jhazmat.2022.128476
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Croplands are experiencing increasing neonicotinoid pollution and ecological health problems, which are especially widely applied in China. However, the large regional scale distribution of neonicotinoids and the key factors have seldom been determined. We show that the total residual concentration of neonicotinoids ranged from 13.4 to 157 ng/g with an average level of 75.8 ng/g and imidacloprid which was the dominant compound ranged from 10.4 to 81.3 ng/g during 2017-2021 in the Yangtze River Delta, China. In comparison, the neonicotinoid residues detected here were mostly higher than those in other regions. We further show that the 1-km spatial resolution cropland coverage (78.0%) and crop type (18.1%) predominantly contributed to the large spatial variation of neonicotinoids after adjusting for the factors including temperature, soil pH, soil moisture, and precipitation via automatic linear regression modeling at the provincial scale. Additional analyses revealed that tea croplands had significantly lowest concentration and fruit fields had the highest level due to the different application methods. Our findings provide new insight into key factors quantifying the high spatial resolved distribution of neonicotinoids and urgently call for reasonable application methods against rapidly growing ecology threats from neonicotinoid pollution in China.
引用
收藏
页数:9
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