Natural Gas Fugitive Emissions Rates Constrained by Global Atmospheric Methane and Ethane

被引:67
作者
Schwietzke, Stefan [1 ,4 ]
Griffin, W. Michael [1 ,2 ]
Matthews, H. Scott [1 ,3 ]
Bruhwiler, Lori M. P. [4 ]
机构
[1] Carnegie Mellon Univ, Dept Engn & Publ Policy, Pittsburgh, PA 15213 USA
[2] Carnegie Mellon Univ, Tepper Sch Business, Pittsburgh, PA 15213 USA
[3] Carnegie Mellon Univ, Dept Civil & Environm Engn, Pittsburgh, PA 15213 USA
[4] NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA
关键词
SHALE GAS; COAL; FOOTPRINT; CHEMISTRY; BUDGET; TREND;
D O I
10.1021/es501204c
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The amount of methane emissions released by the natural gas (NG) industry is a critical and uncertain value for various industry and policy decisions, such as for determining the climate implications of using NG over coal. Previous studies have estimated fugitive emissions rates (FER) the fraction of produced NG (mainly methane and ethane) escaped to the atmosphere between 1 and 9%. Most of these studies rely on few and outdated measurements, and some may represent only temporal/regional NG industry snapshots. This study estimates NG industry representative PER using global atmospheric methane and ethane measurements over three decades, and literature ranges of (i) tracer gas atmospheric lifetimes, (ii) non-NG source estimates, and (iii) fossil fuel fugitive gas hydrocarbon compositions. The modeling suggests an upper bound global average FER of 5% during 2006-2011, and a most likely FER of 2-4% since 2000, trending downward. These results do not account for highly uncertain natural hydrocarbon seepage, which could lower the FER. Further emissions reductions by the NG industry may be needed to ensure climate benefits over coal during the next few decades.
引用
收藏
页码:7714 / 7722
页数:9
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