Pilot verification of a low-tar two-stage coal gasification process with a fluidized bed pyrolyzer and fixed bed gasifier

被引:67
作者
Zeng, Xi [1 ]
Wang, Fang [1 ,2 ]
Li, Hongling [1 ]
Wang, Yin [1 ]
Dong, Li [1 ]
Yu, Jian [1 ]
Xu, Guangwen [1 ]
机构
[1] Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
[2] China Univ Min & Technol, Sch Chem & Environm Engn, Beijing 100083, Peoples R China
基金
美国国家科学基金会;
关键词
Coal; Tar; Two-stage gasification; Fluidized bed; Downdraft fixed bed; BIOMASS GASIFICATION; PRODUCER GAS; TECHNOLOGY; WASTE; PERFORMANCE; DESIGN; ENERGY; CHAR;
D O I
10.1016/j.apenergy.2013.10.052
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
A 50 kg/h autothermal two-stage gasifier, consisting of a fluidized bed (FB) pyrolyzer and a downdraft fixed-bed gasifier, has been designed and built according to our previous laboratory researches. In the experiments, lignite gasification was performed in this innovative two-stage gasifier to demonstrate the process feasibility for clean fuel gas production. The results showed that when keeping the reaction temperatures of the FB pyrolyzer and downdraft fixed bed gasifier respectively at about 860 degrees C and 1100 degrees C, the tar content in the produced fuel gas from the two-stage gasifier was effectively lowered to 84 mg/Nm(3) and the heating value of fuel gas was close to 4.186 MJ/Nm(3). Compared with the tar produced in the FB pyrolyzer, the tar from the downdraft fixed bed gasifier had obviously higher content of light oil components and lower content of heavy components, showing essentially an effective catalytic reforming of tar components by the hot char bed of the downdraft fixed bed gasifier. (C) 2013 Published by Elsevier Ltd.
引用
收藏
页码:9 / 16
页数:8
相关论文
共 32 条
[1]   Mathematical and computational approaches for design of biomass gasification for hydrogen production: A review [J].
Ahmed, Tigabwa Y. ;
Ahmad, Murni M. ;
Yusup, Suzana ;
Inayat, Abrar ;
Khan, Zakir .
RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2012, 16 (04) :2304-2315
[2]   Biomass gasification cogeneration - A review of state of the art technology and near future perspectives [J].
Ahrenfeldt, Jesper ;
Thomsen, Tobias P. ;
Henriksen, Ulrik ;
Clausen, Lasse R. .
APPLIED THERMAL ENGINEERING, 2013, 50 (02) :1407-1417
[3]   Tar reduction in biomass producer gas via mechanical, catalytic and thermal methods: A review [J].
Anis, Samsudin ;
Zainal, Z. A. .
RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2011, 15 (05) :2355-2377
[4]   Process and technological aspects of municipal solid waste gasification. A review [J].
Arena, Umberto .
WASTE MANAGEMENT, 2012, 32 (04) :625-639
[5]   Main routes for the thermo-conversion of biomass into fuels and chemicals. Part 2: Gasification systems [J].
Balat, Mustafa ;
Balat, Mehmet ;
Kirtay, Elif ;
Balat, Havva .
ENERGY CONVERSION AND MANAGEMENT, 2009, 50 (12) :3158-3168
[6]   Characteristics of tar, NOx precursors and their absorption performance with different scrubbing solvents during the pyrolysis of sewage sludge [J].
Chen, Hongfang ;
Namioka, Tomoaki ;
Yoshikawa, Kunio .
APPLIED ENERGY, 2011, 88 (12) :5032-5041
[7]   Matching gasification technologies to coal properties [J].
Collot, AG .
INTERNATIONAL JOURNAL OF COAL GEOLOGY, 2006, 65 (3-4) :191-212
[8]   A review of the primary measures for tar elimination in biomass gasification processes [J].
Devi, L ;
Ptasinski, KJ ;
Janssen, FJJG .
BIOMASS & BIOENERGY, 2003, 24 (02) :125-140
[9]   An advanced biomass gasification technology with integrated catalytic hot gas cleaning Part I. Technology and initial experimental results in a lab-scale facility [J].
Dong, Li ;
Asadullah, Mohammad ;
Zhang, Shu ;
Wang, Xiao-Shan ;
Wu, Hongwei ;
Li, Chun-Zhu .
FUEL, 2013, 108 :409-416
[10]   SIMULATED DISTILLATION BY GAS CHROMATOGRAPHY [J].
GREEN, LE ;
SCHMAUCH, LJ ;
WORMAN, JC .
ANALYTICAL CHEMISTRY, 1964, 36 (08) :1512-&