Smectic liquid crystals in anisotropic colloidal silica gels

被引:27
作者
Liang, D [1 ]
Borthwick, MA
Leheny, RL
机构
[1] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA
[2] MIT, Dept Phys, Cambridge, MA 02139 USA
关键词
D O I
10.1088/0953-8984/16/19/011
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
We report x-ray scattering studies of the smectic liquid crystal octylcyanobiphenol (8CB) confined by strained colloidal silica gels. The gels, comprised of aerosil particles, possess an anisotropic structure that stabilizes long-range nematic order in the liquid crystal while introducing random field effects that disrupt the smectic transition. The short-range smectic correlations that form within this environment are inconsistent with the presence of a topologically ordered state predicted for 3D random field XY systems and are quantitatively like the correlations of smectics confined by isotropic gels. Detailed analysis reveals that the quenched disorder suppresses the anisotropic scaling of the smectic correlation lengths observed in the pure liquid crystal. These results and additional measurements of the smectic-A to smectic-C transition in 4-n-pentylphenylthiol-4'-n-octyloxybenzoate (8S5) indicate that the observed smectic behaviour is dictated by random fields coupling directly to the smectic order while fields coupling to the nematic director play a subordinate role.
引用
收藏
页码:S1989 / S2002
页数:14
相关论文
共 31 条
[1]   DYNAMIC LIGHT-SCATTERING STUDY OF NEMATIC AND SMECTIC-A LIQUID-CRYSTAL ORDERING IN SILICA AEROGEL [J].
BELLINI, T ;
CLARK, NA ;
SCHAEFER, DW .
PHYSICAL REVIEW LETTERS, 1995, 74 (14) :2740-2743
[2]   Universality and scaling in the disordering of a smectic liquid crystal [J].
Bellini, T ;
Radzihovsky, L ;
Toner, J ;
Clark, NA .
SCIENCE, 2001, 294 (5544) :1074-1079
[3]   Light-scattering measurement of the nematic correlation length in a liquid crystal with quenched disorder [J].
Bellini, T ;
Clark, NA ;
Degiorgio, V ;
Mantegazza, F ;
Natale, G .
PHYSICAL REVIEW E, 1998, 57 (03) :2996-3006
[4]   X-RAY-SCATTERING STUDY OF SMECTIC ORDERING IN A SILICA AEROGEL [J].
CLARK, NA ;
BELLINI, T ;
MALZBENDER, RM ;
THOMAS, BN ;
RAPPAPORT, AG ;
MUZNY, CD ;
SCHAEFER, DW ;
HRUBESH, L .
PHYSICAL REVIEW LETTERS, 1993, 71 (21) :3505-3508
[5]   High-resolution x-ray study of the nematic-smectic-A and smectic-A-smectic-C transitions in liquid-crystal-aerosil gels -: art. no. 031706 [J].
Clegg, PS ;
Birgeneau, RJ ;
Park, S ;
Garland, CW ;
Iannacchione, GS ;
Leheny, RL ;
Neubert, ME .
PHYSICAL REVIEW E, 2003, 68 (03) :7
[6]   Effect of a quenched random field on a continuous symmetry breaking transition:: Nematic to smectic-A transition in octyloxycyanobiphenyl-aerosil dispersions -: art. no. 021703 [J].
Clegg, PS ;
Stock, C ;
Birgeneau, RJ ;
Garland, CW ;
Roshi, A ;
Iannacchione, GS .
PHYSICAL REVIEW E, 2003, 67 (02) :13
[7]   Stability of elastic glass phases in random field XY magnets and vortex lattices in type-II superconductors [J].
Fisher, DS .
PHYSICAL REVIEW LETTERS, 1997, 78 (10) :1964-1967
[8]   CRITICAL-BEHAVIOR AT NEMATIC SMECTIC-A PHASE-TRANSITIONS [J].
GARLAND, CW ;
NOUNESIS, G .
PHYSICAL REVIEW E, 1994, 49 (04) :2964-2971
[9]   ELASTIC THEORY OF PINNED FLUX LATTICES [J].
GIAMARCHI, T ;
LEDOUSSAL, P .
PHYSICAL REVIEW LETTERS, 1994, 72 (10) :1530-1533
[10]   Topological defects in the random-field XY model and the pinned vortex lattice to vortex glass transition in type-II superconductors [J].
Gingras, MJP ;
Huse, DA .
PHYSICAL REVIEW B, 1996, 53 (22) :15193-15200