Neel Temperature of Antiferromagnets for Phase Transitions Driven by Spin-wave Interactions

被引:8
作者
Ayuela, Andres [1 ,2 ]
Klein, Douglas J. [3 ]
March, Norman H. [2 ,4 ,5 ]
机构
[1] CFM MPC CSIC UPV EHU, Ctr Fis Mat, San Sebastian 20018, Spain
[2] Univ Pais Vasco UPV EHU, Fac Quim, Dept Fis Mat, Donostia Int Phys Ctr, San Sebastian 20018, Spain
[3] Texas A&M Univ, Galveston, TX 77553 USA
[4] Univ Antwerp, Dept Phys, B-2020 Antwerp, Belgium
[5] Univ Oxford, Oxford, England
关键词
antiferromagnets; transition metal oxides; Neel temperature; magnons; spin-waves; NI2MNGA;
D O I
10.5562/cca2266
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In a recent article,1 a wide variety of phase transitions, with transition (t) temperature T-t, were shown to be usefully characterized by the form k(B)T(t) = E-char exp(-1/vertical bar lambda vertical bar) where vertical bar lambda vertical bar measured the strength of the quasiparticle interactions driving the phase transition. The present article is concerned primarily with antiferromagnets (AFs) having Neel temperature T-N. It is first argued that the characteristic energy E-char can be usefully represented by k(B)theta, where theta is the Curie-Weiss temperature. This assertion is then confronted with experimental data on four insulating transition metal oxides, these being selected as all having the paramagnetic ions on a facecentered cubic lattice. For four of the five theta/T-N is certainly greater than unity, the fifth having the ratio as unity to within experimental error. vertical bar lambda vertical bar is then argued to be related to physical parameters entering a mean field approximation to AFs. Finally, the above insulating Afs are complemented by a brief discussion of a metallic FeRh alloy where, in addition to having itinerant electrons and antiferromagnetism, elevating the temperature leads to a transition from an AF to a ferromagnetic state.
引用
收藏
页码:463 / 467
页数:5
相关论文
共 20 条
[1]   Optimized geometry of the cluster Gd2O3 and proposed antiferromagnetic alignment of f-electron magnetic moment [J].
Ayuela, A. ;
March, N. H. ;
Klein, D. J. .
JOURNAL OF PHYSICAL CHEMISTRY A, 2007, 111 (40) :10162-10165
[2]   Sublattice magnetizations in non-zero magnetic field in an antiferromagnetic infinite-range Ising model [J].
Ayuela, A. ;
Klein, D. J. ;
March, N. H. .
PHYSICS LETTERS A, 2007, 362 (5-6) :468-470
[3]   Ab initio study of tetragonal variants in Ni2MnGa alloy [J].
Ayuela, A ;
Enkovaara, J ;
Nieminen, RM .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2002, 14 (21) :5325-5336
[4]   Structural properties of magnetic Heusler alloys [J].
Ayuela, A ;
Enkovaara, J ;
Ullakko, K ;
Nieminen, RM .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1999, 11 (08) :2017-2026
[5]  
Chaikin PM, 1995, PRINCIPLES CONDENSED
[6]   First-principles calculations of spin spirals in Ni2MnGa and Ni2MnAl -: art. no. 054417 [J].
Enkovaara, J ;
Ayuela, A ;
Jalkanen, J ;
Nordström, L ;
Nieminen, RM .
PHYSICAL REVIEW B, 2003, 67 (05)
[7]   Exchange coupling in transition metal monoxides: Electronic structure calculations [J].
Fischer, Guntram ;
Daene, Markus ;
Ernst, Arthur ;
Bruno, Patrick ;
Lueders, Martin ;
Szotek, Zdzislawa ;
Temmerman, Walter ;
Hergert, Wolfram .
PHYSICAL REVIEW B, 2009, 80 (01)
[8]   Tight-binding theory of manganese and iron oxides [J].
Harrison, Walter A. .
PHYSICAL REVIEW B, 2008, 77 (24)
[9]   Onset of magnetic order in strongly-correlated systems from ab initio electronic structure calculations:: application to transition metal oxides [J].
Hughes, I. D. ;
Daene, M. ;
Ernst, A. ;
Hergert, W. ;
Lueders, M. ;
Staunton, J. B. ;
Szotek, Z. ;
Temmerman, W. M. .
NEW JOURNAL OF PHYSICS, 2008, 10
[10]  
Kiibler J., 2000, THEORY ITINERANT ELE