Contact resistance between bipolar plate and gas diffusion layer in high temperature polymer electrolyte fuel cells

被引:40
作者
Singdeo, Debanand [1 ]
Dey, Tapobrata [1 ]
Ghosh, Prakash C. [1 ]
机构
[1] Indian Inst Technol, Dept Energy Sci & Engn, Bombay 400076, Maharashtra, India
关键词
HT-PEMFC; Contact resistance; Clamping pressure; Carbon paper; Carbon cloth; EFFECTIVE THERMAL-CONDUCTIVITY; CLAMPING PRESSURE; CURRENT COLLECTOR; PERFORMANCE; MODEL; OPTIMIZATION; MEMBRANES; GDL;
D O I
10.1016/j.ijhydene.2013.10.147
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
One of the major contributors to the ohmic loss in fuel cells originates at the interface between adjacent cell components. The compressive pressure used to achieve contact in cells should be carefully estimated to ensure that resistive losses arising from contact behavior remain minimal. In present work, a generic model is developed, capable of estimating contact resistance as a function contact pressure at the interface of graphite bipolar plate and carbon fiber based gas diffusion layer at different temperatures. A good agreement is observed between the results obtained from the model and experiments. Compressive pressure in the ranges of 3-4 MPa is found optimum for achieving low contact resistance. The contact resistance obtained for carbon paper and BPP while using recommended pressure lies between similar to 9 and 4 m Omega cm(2) considering the operating regime of HT-PEMFC (120-180 degrees C). Operating under similar conditions, the contact resistance values for carbon cloth and BPP is similar to 13 to 7 m Omega cm(2). Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:987 / 995
页数:9
相关论文
共 42 条
[1]   Electrical contact resistance between stainless steel bipolar plate and carbon felt in PEFC: A comprehensive study [J].
Andre, Johan ;
Antoni, Laurent ;
Petit, Jean-Pierre ;
De Vito, Eric ;
Montani, Alexandre .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2009, 34 (07) :3125-3133
[2]   Proton-conducting membranes based on benzimidazole polymers for high-temperature PEM fuel cells. A chemical quest [J].
Antonio Asensio, Juan ;
Sanchez, Eduardo M. ;
Gomez-Romero, Pedro .
CHEMICAL SOCIETY REVIEWS, 2010, 39 (08) :3210-3239
[3]   Effect of surface roughness of composite bipolar plates on the contact resistance of a proton exchange membrane fuel cell [J].
Avasarala, Bharat ;
Haldar, Pradeep .
JOURNAL OF POWER SOURCES, 2009, 188 (01) :225-229
[4]   Contact mechanics approach to determine contact surface area between bipolar plates and current collector in proton exchange membrane fuel cells [J].
Barber, M. ;
Sun, T. S. ;
Petrach, E. ;
Wang, X. ;
Zou, Q. .
JOURNAL OF POWER SOURCES, 2008, 185 (02) :1252-1256
[5]   Effect of clamping pressure on the performance of a PEM fuel cell [J].
Chang, W. R. ;
Hwang, J. J. ;
Weng, F. B. ;
Chan, S. H. .
JOURNAL OF POWER SOURCES, 2007, 166 (01) :149-154
[6]   Effects of porosity change of gas diffuser on performance of proton exchange membrane fuel cell [J].
Chu, HS ;
Yeh, C ;
Chen, F .
JOURNAL OF POWER SOURCES, 2003, 123 (01) :1-9
[7]   Study of contact resistance at the electrode-interconnect interfaces in planar type Solid Oxide Fuel Cells [J].
Dey, Tapobrata ;
Singdeo, Debanand ;
Bose, Manaswita ;
Basu, Rajendra N. ;
Ghosh, Prakash C. .
JOURNAL OF POWER SOURCES, 2013, 233 :290-298
[8]   Bipolar plate thermal response to PEM fuel cell stack compressive load [J].
Fekrazad, N. ;
Bergman, T. L. .
JOURNAL OF HEAT TRANSFER-TRANSACTIONS OF THE ASME, 2008, 130 (06)
[9]   CONTACT OF NOMINALLY FLAT SURFACES [J].
GREENWOOD, JA ;
WILLIAMSON, JB .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1966, 295 (1442) :300-+
[10]  
Holm R, 2000, Electric contacts: theory and applications, DOI DOI 10.1007/978-3-662-06688-1