Laser ionization mass spectrometry at 55: Quo Vadis?

被引：24

作者：

Azov, Vladimir A. ^{[1
]}

Mueller, Larissa ^{[2
]}

Makarov, Alexander A. ^{[2
,3
]}

机构：

[1] Univ Free State, Dept Chem, POB 339, ZA-9300 Bloemfontein, South Africa

[2] Thermo Fisher Sci GmbH, D-28199 Bremen, Germany

[3] Univ Utrecht, Utrecht Inst Pharmaceut Sci, Bijvoet Ctr Biomol Res, Biomol Mass Spectrometry & Prote, Utrecht, Netherlands

来源：

MASS SPECTROMETRY REVIEWS | 2022年 / 41卷 / 01期

关键词：

depth profiling; elemental analysis; laser ablation; laser ionization; mass spectrometry; mass spectrometry imaging; surface analysis; ATMOSPHERIC-PRESSURE PHOTOIONIZATION; TRANSITION-METAL COMPOUNDS; ALKALINE-EARTH CHROMATE; LA-ICP-MS; IN-SITU; DESORPTION IONIZATION; ELEMENTAL ANALYSIS; ELECTROSPRAY-IONIZATION; PERFORMANCE EVALUATION; CHEMICAL-ANALYSIS;

D O I：

10.1002/mas.21669

中图分类号：

O433 [光谱学];

学科分类号：

0703 ; 070302 ;

摘要：

Laser ionization mass spectrometry (LIMS) was one of the first practical methods developed for in situ analysis of the surfaces of solid samples. This review will encompass several aspects related to this analytical method. First, we will discuss the process of laser ionization, the influence of the laser type on its performance, and imaging capabilities of this method. In the second chapter, we will follow the historic development of LIMS instrumentation. After a brief overview of the first-generation instruments developed in 1960-1990 years, we will discuss in detail more recent designs, which appeared during the last 2-3 decades. In the last part of our review, we will cover the recent applications of LIMS for surface analysis. These applications include various types of analyses of solid inorganic, organic, and heterogeneous samples, often in combination with depth profiling and imaging capability.

引用

页码：100 / 151

页数：52

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