Stimulated Emission and Lasing from CdSe/CdS/ZnS Core-Multi-Shell Quantum Dots by Simultaneous Three-Photon Absorption

被引:172
作者
Wang, Yue [1 ]
Van Duong Ta [1 ]
Gao, Yuan [1 ]
He, Ting Chao [1 ]
Chen, Rui [1 ]
Mutlugun, Evren [2 ]
Demir, Hilmi Volkan [2 ,3 ,4 ,5 ]
Sun, Han Dong [1 ,3 ]
机构
[1] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore
[2] Nanyang Technol Univ, Sch Elect & Elect Engn, Luminous Ctr Excellence Semicond Lighting & Displ, Singapore 639798, Singapore
[3] Nanyang Technol Univ, CDPT, Singapore 637371, Singapore
[4] Bilkent Univ, Dept Phys, Dept Elect & Elect Engn, TR-06533 Bilkent, Turkey
[5] Bilkent Univ, UNAM Natl Nanotechnol Res Ctr, Bilkent, Turkey
基金
新加坡国家研究基金会;
关键词
lasing; quantum dots; multi-photon excitation; Auger recombination; AMPLIFIED SPONTANEOUS EMISSION; OPTICAL GAIN; SEMICONDUCTOR NANOCRYSTALS; CDSE; LIGHT; MICROSCOPY;
D O I
10.1002/adma.201305125
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Three-photon pumped stimulated emission and coherent random lasing from colloidal CdSe/CdS/ZnS core-multishell quantum dots are achieved for the first time. These results can offer new possibilities in biology and photonics, as well as at their intersection of biophotonics. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:2954 / 2961
页数:8
相关论文
共 54 条
  • [1] Single-step synthesis of quantum dots with chemical composition gradients
    Bae, Wan Ki
    Char, Kookheon
    Hur, Hyuck
    Lee, Seonghoon
    [J]. CHEMISTRY OF MATERIALS, 2008, 20 (02) : 531 - 539
  • [2] Spatial confinement of laser light in active random media
    Cao, H
    Xu, JY
    Zhang, DZ
    Chang, SH
    Ho, ST
    Seelig, EW
    Liu, X
    Chang, RPH
    [J]. PHYSICAL REVIEW LETTERS, 2000, 84 (24) : 5584 - 5587
  • [3] Random laser action in semiconductor powder
    Cao, H
    Zhao, YG
    Ho, ST
    Seelig, EW
    Wang, QH
    Chang, RPH
    [J]. PHYSICAL REVIEW LETTERS, 1999, 82 (11) : 2278 - 2281
  • [4] Lasing in random media
    Cao, H
    [J]. WAVES IN RANDOM MEDIA, 2003, 13 (03): : R1 - R39
  • [5] FRET-assisted laser emission in colloidal suspensions of dye-doped latex nanoparticles
    Cerdan, Luis
    Enciso, Eduardo
    Martin, Virginia
    Banuelos, Jorge
    Lopez-Arbeloa, Inigo
    Costela, Angel
    Garcia-Moreno, Inmaculada
    [J]. NATURE PHOTONICS, 2012, 6 (09) : 621 - 626
  • [6] Exciton Localization and Optical Properties Improvement in Nanocrystal-Embedded ZnO Core-Shell Nanowires
    Chen, Rui
    Ye, Quan-Lin
    He, Tingchao
    Van Duong Ta
    Ying, Yongjun
    Tay, Yee Yan
    Wu, Tom
    Sun, Handong
    [J]. NANO LETTERS, 2013, 13 (02) : 734 - 739
  • [7] Three-photon excited band edge and trap emission of CdS semiconductor nanocrystals
    Chon, JWM
    Gu, M
    Bullen, C
    Mulvaney, P
    [J]. APPLIED PHYSICS LETTERS, 2004, 84 (22) : 4472 - 4474
  • [8] Cooney R.R., 2009, Journal of Chemical Physics, P131
  • [9] Cooney R. R., 2009, PHYS REV LETT, P102
  • [10] Dang C, 2012, NAT NANOTECHNOL, V7, P335, DOI [10.1038/NNANO.2012.61, 10.1038/nnano.2012.61]