Coordination-Driven Polymerization of Supramolecular Nanocages

被引：82

作者：

Niu, Zheng ^{[1
,2
,3
]}

Fang, Sheng ^{[1
,2
]}

Liu, Xiao ^{[1
,2
]}

Ma, Jian-Gong ^{[1
,2
]}

Ma, Shengqian ^{[3
]}

Cheng, Peng ^{[1
,2
]}

机构：

[1] Nankai Univ, Dept Chem, Key Lab Adv Energy Mat Chem MOE, Tianjin 300071, Peoples R China

[2] Nankai Univ, Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300071, Peoples R China

[3] Univ S Florida, Dept Chem, Tampa, FL 33620 USA

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2015年 / 137卷 / 47期

关键词：

METAL-ORGANIC POLYHEDRA; PORE-SIZE; CAGES; DISCRETE; FRAMEWORKS; SUPERCONTAINERS; NANOSTRUCTURES; TRANSFORMATION; CONVERSION; ASSEMBLIES;

D O I：

10.1021/jacs.5b10815

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Controlled assembly of OD supramolecular nanocages into 2D or 3D architectures has been demonstrated for the first time via a coordination-driven polymerization approach, and the conversion from a 2D to 3D supramolecular architecture has also been successfully achieved via a temperature-induced crystal transformation. The boost of dimensionality for the supramolecular architecture has led to steady yet remarkable enhancement of properties, as reflected from the gas adsorption studies.

引用

页码：14873 / 14876

页数：4

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