Asian emissions in 2006 for the NASA INTEX-B mission

被引:1704
作者
Zhang, Q. [1 ,2 ]
Streets, D. G. [1 ]
Carmichael, G. R. [3 ]
He, K. B. [2 ]
Huo, H. [4 ]
Kannari, A.
Klimont, Z. [5 ]
Park, I. S. [6 ]
Reddy, S. [7 ]
Fu, J. S. [8 ]
Chen, D. [2 ]
Duan, L. [2 ]
Lei, Y. [2 ]
Wang, L. T. [2 ]
Yao, Z. L. [2 ]
机构
[1] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA
[2] Tsinghua Univ, Dept Environm Sci & Engn, Beijing 100084, Peoples R China
[3] Univ Iowa, Ctr Global & Reg Environm Res, Iowa City, IA 52242 USA
[4] Argonne Natl Lab, Ctr Transportat Res, Argonne, IL 60439 USA
[5] Int Inst Appl Syst Anal, A-2361 Laxenburg, Austria
[6] Hankuk Univ Foreign Studies, Dept Environm, Yongin, South Korea
[7] Hadley Ctr, UK Met Off, Exeter EX1 3PB, Devon, England
[8] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA
关键词
VOLATILE ORGANIC-COMPOUNDS; SIMULATED TROPOSPHERIC NO2; SULFUR-DIOXIDE EMISSIONS; PACIFIC TRACE-P; EAST-ASIA; CARBONACEOUS PARTICLES; SURFACE OBSERVATIONS; CHEMICAL EVOLUTION; ENERGY-CONSUMPTION; OZONE POLLUTION;
D O I
10.5194/acp-9-5131-2009
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A new inventory of air pollutant emissions in Asia in the year 2006 is developed to support the Intercontinental Chemical Transport Experiment-Phase B (INTEX-B) funded by the National Aeronautics and Space Administration (NASA). Emissions are estimated for all major anthropogenic sources, excluding biomass burning. We estimate total Asian anthropogenic emissions in the year 2006 as follows: 47.1 Tg SO2, 36.7 Tg NOx, 298.2 Tg CO, 54.6 Tg NMVOC, 29.2 Tg PM10, 22.2 Tg PM2.5, 2.97 Tg BC, and 6.57 Tg OC. We emphasize emissions from China because they dominate the Asia pollutant outflow to the Pacific and the increase of emissions from China since 2000 is of great concern. We have implemented a series of improved methodologies to gain a better understanding of emissions from China, including a detailed technology-based approach, a dynamic methodology representing rapid technology renewal, critical examination of energy statistics, and a new scheme of NMVOC speciation for model-ready emissions. We estimate China's anthropogenic emissions in the year 2006 to be as follows: 31.0 Tg SO2, 20.8 Tg NOx, 166.9 Tg CO, 23.2 Tg NMVOC, 18.2 Tg PM10, 13.3 Tg PM2.5, 1.8 Tg BC, and 3.2 Tg OC. We have also estimated 2001 emissions for China using the same methodology and found that all species show an increasing trend during 2001-2006: 36% increase for SO2, 55% for NOx, 18% for CO, 29% for VOC, 13% for PM10, and 14% for PM2.5, BC, and OC. Emissions are gridded at a resolution of 30 minx30 min and can be accessed at our web site (< a href='http://mic.greenresource.cn/intex-b2006' target='_blank'> http://mic.greenresource.cn/intex-b2006 </a >).
引用
收藏
页码:5131 / 5153
页数:23
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