Highly efficient and stable white LEDs based on pure red narrow bandwidth emission triangular carbon quantum dots for wide-color gamut backlight displays

被引:131
作者
Yuan, Fanglong [1 ]
He, Ping [1 ]
Xi, Zifan [1 ]
Li, Xiaohong [1 ]
Li, Yunchao [1 ]
Zhong, Haizheng [2 ]
Fan, Louzhen [1 ]
Yang, Shihe [3 ]
机构
[1] Beijing Normal Univ, Coll Chem, Beijing 100875, Peoples R China
[2] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing Key Lab Nanophoton & Ultrafine Optoelect, Beijing 100081, Peoples R China
[3] Peking Univ, Shenzhen Grad Sch, Sch Chem Biol & Biotechnol, Guangdong Key Lab Nanomicro Mat Res, Shenzhen 518055, Peoples R China
基金
中国国家自然科学基金;
关键词
pure red; carbon quantum dots; white light-emitting diodes; wide-color gamut; highly efficient; LIGHT-EMITTING-DIODES; HIGH-PERFORMANCE; GREEN; LUMINESCENT; PHOTOLUMINESCENCE;
D O I
10.1007/s12274-019-2420-x
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
High-performance white light-emitting diodes (WLEDs) hold great potential for the next-generation backlight display applications. However, achieving highly efficient and stable WLEDs with wide-color-gamut has remained a formidable goal. Reported here is the first example of pure red narrow bandwidth emission triangular CQDs (PR-NBE-T-CQDs) with photoluminescence peaking at 610 nm. The PR-NBE-T-CQDs synthesized from resorcinol show high quantum yield (QY) of 72% with small full width at half maximum of 33 nm. By simply controlling the reaction time, pure green (PG-) NBE-T-CQDs with high QY of 75% were also obtained. Highly efficient and stable WLEDs with wide-color-gamut based on PR- and PG-NBE-T-CQDs was achieved. This WLED showed a remarkable wide-color gamut of 110% NTSC and high power efficiency of 86.5 lumens per Watt. Furthermore, such WLEDs demonstrate outstanding stability. This work will set the stage for developing highly efficient, low cost and environment-friendly WLEDs based on CQDs for the next-generation wide-color gamut backlight displays.
引用
收藏
页码:1669 / 1674
页数:6
相关论文
共 40 条
[1]  
[Anonymous], 2016, Angew. Chem.
[2]   Photoluminescence-Tunable Carbon Nanodots: Surface-State Energy-Gap Tuning [J].
Bao, Lei ;
Liu, Cui ;
Zhang, Zhi-Ling ;
Pang, Dai-Wen .
ADVANCED MATERIALS, 2015, 27 (10) :1663-+
[3]   Quantum-dot optoelectronic devices [J].
Bhattacharya, Pallab ;
Mi, Zetian .
PROCEEDINGS OF THE IEEE, 2007, 95 (09) :1723-1740
[4]   Recent Advances on Quantum-Dot-Enhanced Liquid-Crystal Displays [J].
Chen, Haiwei ;
He, Juan ;
Wu, Shin-Tson .
IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, 2017, 23 (05)
[5]   Solvothermal Synthesis of High-Quality All-Inorganic Cesium Lead Halide Perovskite Nanocrystals: From Nanocube to Ultrathin Nanowire [J].
Chen, Min ;
Zou, Yatao ;
Wu, Linzhong ;
Pan, Qi ;
Yang, Di ;
Hu, Huicheng ;
Tan, Yeshu ;
Zhong, Qixuan ;
Xu, Yong ;
Liu, Haiyu ;
Sun, Baoquan ;
Zhang, Qiao .
ADVANCED FUNCTIONAL MATERIALS, 2017, 27 (23)
[6]   A Self-Quenching-Resistant Carbon-Dot Powder with Tunable Solid-State Fluorescence and Construction of Dual-Fluorescence Morphologies for White Light-Emission [J].
Chen, Yonghao ;
Zheng, Mingtao ;
Xiao, Yong ;
Dong, Hanwu ;
Zhang, Haoran ;
Zhuang, Jianle ;
Hu, Hang ;
Lei, Bingfu ;
Liu, Yingliang .
ADVANCED MATERIALS, 2016, 28 (02) :312-318
[7]   Electroluminescence from single monolayers of nanocrystals in molecular organic devices [J].
Coe, S ;
Woo, WK ;
Bawendi, M ;
Bulovic, V .
NATURE, 2002, 420 (6917) :800-803
[8]   Quantum-Dot Light-Emitting Diodes for Large-Area Displays: Towards the Dawn of Commercialization [J].
Dai, Xingliang ;
Deng, Yunzhou ;
Peng, Xiaogang ;
Jin, Yizheng .
ADVANCED MATERIALS, 2017, 29 (14)
[9]   Solution-processed, high-performance light-emitting diodes based on quantum dots [J].
Dai, Xingliang ;
Zhang, Zhenxing ;
Jin, Yizheng ;
Niu, Yuan ;
Cao, Hujia ;
Liang, Xiaoyong ;
Chen, Liwei ;
Wang, Jianpu ;
Peng, Xiaogang .
NATURE, 2014, 515 (7525) :96-99
[10]   White-Light-Emitting Diodes with Quantum Dot Color Converters for Display Backlights [J].
Jang, Eunjoo ;
Jun, Shinae ;
Jang, Hyosook ;
Llim, Jungeun ;
Kim, Byungki ;
Kim, Younghwan .
ADVANCED MATERIALS, 2010, 22 (28) :3076-3080