Enhanced Visible Light Photocatalytic Degradation of Rhodamine B by Bi2WO6-Reduced Graphene Oxide Composites Prepared via Microwave-Assisted Method

被引:1
作者
Yu, Kai [2 ]
Liu, Xinjuan [1 ,3 ]
Li, Jinliang [2 ]
Chen, Taiqiang [2 ]
Sun, Zhuo [2 ]
Sun, Chang Q. [1 ]
机构
[1] China Jiliang Univ, Coll Mat Sci & Engn, Ctr Coordinat Bond & Elect Engn, Hangzhou 310018, Peoples R China
[2] E China Normal Univ, Dept Phys, Engn Res Ctr Nanophoton & Adv Instrument, Minist Educ, Shanghai 200062, Peoples R China
[3] Shanghai Nanotechnl Promot Ctr, Shanghai 200237, Peoples R China
基金
中国博士后科学基金;
关键词
Microwave-Assisted Method; Bi2WO6; Reduced Graphene Oxide; Photocatalysis; Rhodamine B; SENSITIZED SOLAR-CELLS; SELECTIVE OXIDATION; CARBON NANOTUBE; ANATASE TIO2; BI2WO6; PERFORMANCE; NANOCOMPOSITES; SEMICONDUCTOR; FABRICATION; REDUCTION;
D O I
10.1166/nnl.2014.1816
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Bi2WO6-reduced graphene oxide (RGO) composites were successfully synthesized via microwave-assisted reduction of graphite oxide in Bi2WO6 precursor solution using a microwave system. Their morphologies, structures, and photocatalytic performance in the degradation of Rhodamine B (RhB) were characterized by scanning electron microscopy, transmission electron microscopy, X-ray diffraction, UV-vis absorption spectroscopy, and electrochemical impedance spectroscopy, respectively. The results show that the RGO addition can enhance the photocatalytic performance of Bi2WO6. Bi2WO6-RGO composite with 0.8 wt% RGO achieves a maximum RhB degradation rate at 240 min under visible light irradiation, much higher than that for Bi2WO6 (72%). The enhanced photocatalytic performance is ascribed to the increased light absorption and the reduction in electron-hole pair recombination in Bi2WO6 with the introduction of RGO.
引用
收藏
页码:666 / 671
页数:6
相关论文
共 51 条
[21]   Homogeneous core/shell Bi2WO6 spherical photocatalysts: their controlled synthesis and enhanced visible-light photocatalytic performances [J].
Mao, Chaochao ;
Li, Maolin ;
Fang, Zhiguo ;
Meng, Fanli ;
Qu, Xiaoni ;
Liu, Yanping ;
Wang, Mengjiao ;
Zhang, Ji ;
Shi, Zhan ;
Guo, Xiaohui .
RSC ADVANCES, 2013, 3 (18) :6631-6639
[22]   Enhanced photocatalytic performance of Bi2WO6 by graphene supporter as charge transfer channel [J].
Min, Yu-Lin ;
Zhang, Kan ;
Chen, You-Cun ;
Zhang, Yuan-Guang .
SEPARATION AND PURIFICATION TECHNOLOGY, 2012, 86 :98-105
[23]   Microwave assisted synthesis -: a critical technology overview [J].
Nüchter, M ;
Ondruschka, B ;
Bonrath, W ;
Gum, A .
GREEN CHEMISTRY, 2004, 6 (03) :128-141
[24]   Toward rapid, "green", predictable microwave-assisted synthesis [J].
Roberts, BA ;
Strauss, CR .
ACCOUNTS OF CHEMICAL RESEARCH, 2005, 38 (08) :653-661
[25]   Solvothermal Preparation of ZnO/Graphene Nanocomposites and Its Photocatalytic Properties [J].
Saranya, M. ;
Garg, Srishti ;
Singh, Iksha ;
Ramachandran, R. ;
Santhosh, C. ;
Harish, C. ;
Vanchinathan, T. Mudaliar ;
Chandra, M. Bhanu ;
Grace, A. Nirmala .
NANOSCIENCE AND NANOTECHNOLOGY LETTERS, 2013, 5 (03) :349-354
[26]  
Sun SW, 2012, INT J OFFSHORE POLAR, V22, P1
[27]   Bi2WO6 Quantum Dots Decorated Reduced Graphene Oxide: Improved Charge Separation and Enhanced Photoconversion Efficiency [J].
Sun, Songmei ;
Wang, Wenzhong ;
Zhang, Ling .
JOURNAL OF PHYSICAL CHEMISTRY C, 2013, 117 (18) :9113-9120
[28]   A high-performance Bi2WO6-graphene photocatalyst for visible light-induced H2 and O2 generation [J].
Sun, Zhihua ;
Guo, Jingjing ;
Zhu, Shenmin ;
Mao, Lin ;
Ma, Jun ;
Zhang, Di .
NANOSCALE, 2014, 6 (04) :2186-2193
[29]   Photocatalytic Activity of Au Nanoparticles Synthesized by Piper pedicellatum C.DC Fruits [J].
Tamuly, Chandan ;
Hazarika, Moushumi ;
Das, Manash R. ;
Bordoloi, Manob Jyoti .
NANOSCIENCE AND NANOTECHNOLOGY LETTERS, 2013, 5 (07) :758-764
[30]   A Bi2WO6-Based Hybrid Photocatalyst with Broad Spectrum Photocatalytic Properties under UV, Visible, and Near-Infrared Irradiation [J].
Tian, Jian ;
Sang, Yuanhua ;
Yu, Guangwei ;
Jiang, Huaidong ;
Mu, Xiaoning ;
Liu, Hong .
ADVANCED MATERIALS, 2013, 25 (36) :5075-5080