Emerging Pt-based electrocatalysts with highly open nanoarchitectures for boosting oxygen reduction reaction

被引：314

作者：

Li, Cuiling ^{[1
]}

Tan, Haibo ^{[2
,3
]}

Lin, Jianjian ^{[1
]}

Luo, Xiliang ^{[1
]}

Wang, Shengping ^{[4
]}

You, Jungmok ^{[5
]}

Kang, Yong-Hook ^{[6
]}

Bando, Yoshio ^{[2
]}

Yamauchi, Yusuke ^{[5
,7
,8
]}

Kim, Jeonghun ^{[7
,8
]}

机构：

[1] Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Qingdao 266042, Peoples R China

[2] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton MANA, 1-1 Namiki, Tsukuba, Ibaraki 3050044, Japan

[3] Waseda Univ, Fac Sci & Engn, Shinjuku Ku, 3-4-1 Okubo, Tokyo 1698555, Japan

[4] China Univ Geosci, Fac Mat Sci & Chem, Wuhan 430074, Hubei, Peoples R China

[5] Kyung Hee Univ, Dept Plant & Environm New Resources, 1732 Deogyeong Daero, Yongin 446701, Gyeonggi Do, South Korea

[6] Dongguk Univ Seoul, Dept Energy & Mat Engn, 30,Pildong Ro 1 Gil, Seoul, South Korea

[7] Univ Queensland, Sch Chem Engn, Brisbane, Qld 4072, Australia

[8] Univ Queensland, AIBN, Brisbane, Qld 4072, Australia

来源：

NANO TODAY | 2018年 / 21卷

基金：

澳大利亚研究理事会; 新加坡国家研究基金会;

关键词：

Pt-based electrocatalysts; Nanoarchitecture; Oxygen reduction reaction (ORR); Metal nanomaterials; Fuel cell; Open construction; HIGH-INDEX FACETS; MESOPOROUS PLATINUM NANOSPHERES; SIZE-CONTROLLED SYNTHESIS; ELECTROCHEMICAL SYNTHESIS; MEDIATED SYNTHESIS; ENHANCED ACTIVITY; FILMS; CATALYSTS; NANOCRYSTALS; NANOWIRES;

D O I：

10.1016/j.nantod.2018.06.005

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Developing highly efficient and stable platinum (Pt)-based electrocatalysts for oxygen reduction reaction (ORR) is the most essential step toward the commercialization of fuel cells. Highly accessible reactive surfaces play a key role in boosting ORR for superior fuel cell performance due to the adequate exposure of the active surfaces and the feasible mass transport. Herein, we begin with a brief introduction to the design principles for an effective ORR electrocatalyst, which could plausibly possess high activity and durability at the same time. Corresponding with the requirements, the recent progress of rational design based on nanoarchitecture, synthesis, and electrochemical performances of Pt -based electrocatalysts with open construction is reviewed and explained accordingly. (C) 2018 Elsevier Ltd. All rights reserved.

引用

页码：91 / 105

页数：15

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