Dependence of tunneling ionization and harmonic generation on the structure of molecules by short intense laser pulses

被引：22

作者：

Lin, C. D. ^{[1
]}

Tong, X. M.

机构：

[1] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA

[2] Univ Tsukuba, Grad Sch Pure & Appl Sci, Inst Mat Sci, Tsukuba, Ibaraki 3058573, Japan

[3] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058577, Japan

来源：

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY | 2006年 / 182卷 / 03期

关键词：

tunneling ionization rates; harmonic generation; attosecond pulses; vibrational wave packet; molecular alignment;

D O I：

10.1016/j.jphotochem.2006.04.027

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We illustrate how the sub-10fs lasers and attosecond XUV pulses can be used to probe the structure of molecules. Experimental results of the alignment dependence of the ionization rates and the high-order harmonic generation yields are shown to reflect the structure of the highest occupied molecular orbital. We also show that the vibrational wave packet of simple molecules can be mapped accurately, including the broadening and interference, by using attosecond light pulses. (c) 2006 Elsevier B.V. All rights reserved.

引用

页码：213 / 219

页数：7

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