Carbon nanotube (CNT) metal composites exhibit greatly reduced radiation damage

被引:25
作者
Cao, Penghui [2 ]
So, Kang Pyo [1 ]
Yang, Yang [1 ,6 ]
Park, Jong Gil [3 ]
Li, Mingda [1 ]
Yan, Long [4 ]
Hu, Jing [5 ]
Kirk, Mark [5 ]
Li, Meimei [5 ]
Lee, Young Hee [3 ]
Short, Michael P. [1 ]
Li, Ju [1 ,7 ]
机构
[1] MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA
[2] Univ Calif Irvine, Dept Mech & Aerosp Engn, Irvine, CA 92697 USA
[3] Sungkyunkwan Univ, Inst Basic Sci, IBS Ctr Integrated Nanostruct Phys, Seoul 440746, South Korea
[4] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China
[5] Argonne Natl Lab, Nucl Sci & Engn Div, Lemont, IL 60439 USA
[6] Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Mol Foundry, 67 Cyclotron Rd, Berkeley, CA 94720 USA
[7] MIT, Dept Mat Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA
关键词
ion irradiation; IVEM; carbon nanotubes; nuclear materials; in situ; defects; MECHANISMS; REDUCTION; MIGRATION; DYNAMICS; ENERGY;
D O I
10.1016/j.actamat.2020.116483
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Radiation damage of structural materials leads to mechanical property degradation, eventually inducing failure. Secondary-phase dispersoids or other defect sinks are often added to materials to boost their radiation resistance. We demonstrate that a metal composite made by adding 1D carbon nanotubes (CNTs) to aluminum (Al) exhibits superior radiation resistance. In situ ion irradiation with transmission electron microscopy (TEM) and atomistic simulations together reveal the mechanisms of rapid defect migration to CNTs, facilitating defect recombination and enhancing radiation tolerance. The origin of this effect is an evolving stress gradient in the Al matrix resulting from CNT transformation under irradiation, and the stability of resulting carbides. Extreme value statistics of large defect behavior in our simulations highlight the role of CNTs in reducing accumulated damage. This approach to controlling defect migration represents a promising opportunity to enhance the radiation resistance of nuclear materials without detrimental effects. (C) 2020 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
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页数:8
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