Seasonal characteristics of aerosol vertical structure and autumn enhancement of non-spherical particle over the semi-arid region of northwest China

被引:14
作者
Zhou, Tian [1 ]
Xie, Hailing [1 ]
Jiang, Tao [2 ]
Huang, Jianping [1 ]
Bi, Jianrong [1 ]
Huang, Zhongwei [1 ]
Shi, Jinsen [1 ]
机构
[1] Lanzhou Univ, Coll Atmospher Sci, Minist Educ, Key Lab Semiarid Climate Change, Lanzhou 730000, Peoples R China
[2] Natl Univ Def Technol, Coll Meteorol & Oceanog, Changsha 410000, Peoples R China
基金
美国国家科学基金会;
关键词
Seasonal characteristics; Aerosol vertical structure; Non-spherical particle enhancement; Lidar; YANGTZE-RIVER DELTA; GROUND-BASED LIDAR; OPTICAL-PROPERTIES; DUST AEROSOL; ANTHROPOGENIC DUST; POLLUTION EVENTS; LOESS PLATEAU; CLIMATE; ABSORPTION; LAYER;
D O I
10.1016/j.atmosenv.2020.117912
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Assessments of the effects of aerosols on the climate and environment still feature large uncertainties, and a better understanding of the spatiotemporal variation in these effects is needed. In this study, coincident obser-vations of ground-based lidar and sun photometer measurements from March 2010 to February 2011 were selected to examine the sensible seasonal characteristics of the aerosol vertical structure and the potential variations of aerosol properties before and during the wintertime heating period at SACOL (Semi-Arid Climate and Environment Observatory of Lanzhou University, 35.946 degrees N, 104.137 degrees E, 1961 m ASL), northwest of China. Our results suggest that the aerosol behavior during a year can be roughly divided into two major periods: the non spherical particle dominated period and the spherical particle dominated period based on the depolarization ratio, or the dust-dominated period (spring and winter) and the non-dust-dominated period (summer and autumn) based on the aerosol angstrom exponent. The height and width of peak of aerosol scale height frequency distribution show the distribution of aerosol layers in summer is highest, then followed by spring, autumn and winter. The depolarization ratios at different heights in spring are higher than those in other seasons. A similar distribution of extinction coefficients above 2 km can be seen in four seasons, but relatively large differences exist below 2 km, especially within 1 km. The increase of the extinction coefficient is observed near surface in November 2010 with a sharp increase in depolarization ratio which is induced by the rising contribution of the dust events (up to 13%) and the mixed type aerosols (70%). These results not only provide detailed characteristics of aerosol variation over the SACOL region, but also remind us to take into account the potential contribution of dust aerosol to the severe regional air pollution during the wintertime heating period.
引用
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页数:10
相关论文
共 69 条
[1]  
[Anonymous], 1998, Principals governing IPCC work
[2]   Measurement of scattering and absorption properties of dust aerosol in a Gobi farmland region of northwestern China - a potential anthropogenic influence [J].
Bi, Jianrong ;
Huang, Jianping ;
Shi, Jinsen ;
Hu, Zhiyuan ;
Zhou, Tian ;
Zhang, Guolong ;
Huang, Zhongwei ;
Wang, Xin ;
Jin, Hongchun .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2017, 17 (12) :7775-7792
[3]   Comparison of key absorption and optical properties between pure and transported anthropogenic dust over East and Central Asia [J].
Bi, Jianrong ;
Huang, Jianping ;
Holben, Brent ;
Zhang, Guolong .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2016, 16 (24) :15501-15516
[4]   Aerosol transport over the Andes from the Amazon Basin to the remote Pacific Ocean: A multiyear CALIOP assessment [J].
Bourgeois, Quentin ;
Ekman, Annica M. L. ;
Krejci, Radovan .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2015, 120 (16) :8411-8425
[5]   Statistics of aerosol extinction coefficient profiles and optical depth using lidar measurement over Lanzhou, China since 2005-2008 [J].
Cao, X. ;
Wang, Z. ;
Tian, P. ;
Wang, J. ;
Zhang, L. ;
Quan, X. .
JOURNAL OF QUANTITATIVE SPECTROSCOPY & RADIATIVE TRANSFER, 2013, 122 :150-154
[6]   CLIMATE FORCING BY ANTHROPOGENIC AEROSOLS [J].
CHARLSON, RJ ;
SCHWARTZ, SE ;
HALES, JM ;
CESS, RD ;
COAKLEY, JA ;
HANSEN, JE ;
HOFMANN, DJ .
SCIENCE, 1992, 255 (5043) :423-430
[7]   Study on the aerosol optical properties and their relationship with aerosol chemical compositions over three regional background stations in China [J].
Che, Huizheng ;
Yang, Zhifeng ;
Zhang, Xiaoye ;
Zhu, Chize ;
Ma, Qiangli ;
Zhou, Huaigang ;
Wang, Peng .
ATMOSPHERIC ENVIRONMENT, 2009, 43 (05) :1093-1099
[8]  
Chen Z., 2014, EPJ WEB C, V119, P24008
[9]   Relationship between Aerosol Optical Depth and Particulate Matter over Singapore: Effects of Aerosol Vertical Distributions [J].
Chew, Boon Ning ;
Campbell, James R. ;
Hyer, Edward J. ;
Salinas, Santo V. ;
Reid, Jeffrey S. ;
Welton, Ellsworth J. ;
Holben, Brent N. ;
Liew, Soo Chin .
AEROSOL AND AIR QUALITY RESEARCH, 2016, 16 (11) :2818-2830
[10]   Sensitivity of aerosol direct radiative forcing to aerosol vertical profile [J].
Choi, Jung-Ok ;
Chung, Chul E. .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2014, 66