Optical second harmonic generation in centrosymmetric antiferro magnetic NiO

被引：2
|
作者：
Fiebig, M [1 ]
Fröhlich, D [1 ]
Lottermoser, T [1 ]
Pavlov, VV [1 ]
Pisarev, RV [1 ]
Weber, HJ [1 ]
机构：
[1] Univ Dortmund, Inst Phys, D-44221 Dortmund, Germany
来源：
XI FEOFILOV SYMPOSIUM ON SPECTROSCOPY OF CRYSTALS ACTIVATED BY RARE-EARTH AND TRANSITION METAL IONS | 2002年 / 4766卷
关键词：
magnetic structure; nonlinear optics; second harmonic generation; centrosymmetry; NiO; magneto-optics; domains; antiferromagnetism; transition metals;
D O I：
10.1117/12.475340
中图分类号：
TM [电工技术]; TN [电子技术、通信技术];
学科分类号：
0808 ; 0809 ;
摘要：
Optical second harmonic generation (SHG) in NiO in spectroscopy and topography experiments reveals a pronounced signal below the Neel temperature which couples quadratically to the antiferromagnetic order parameter. The SH process originates in combined magnetic-dipole and electric-dipole transitions between the (3d)(8) levels of the Ni2+ ion in the crystal field. It is greatly enhanced by being resonant both in the incoming and the outgoing light waves. The polarization dependence reveals a sensitivity of the SH process to both T and S domains which are investigated in imaging experiments.
引用
收藏
页码：238 / 247
页数：10
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