Graphene-Based Advanced Membrane Applications in Organic Solvent Nanofiltration

被引:113
作者
Nie, Lina [1 ]
Chuah, Chong Yang [2 ]
Bae, Tae-Hyun [3 ]
Lee, Jong-Min [1 ]
机构
[1] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore
[2] Nanyang Technol Univ, Nanyang Environm & Water Res Inst, Singapore Membrane Technol Ctr, Singapore 637141, Singapore
[3] Korea Adv Inst Sci & Technol KAIST, Dept Chem & Biomed Engn, Daejeon 305338, South Korea
关键词
graphene‐ based membrane; graphene oxide; membrane; organic solvent nanofiltration; upper bound; MIXED-MATRIX MEMBRANES; LINKED POLYBENZIMIDAZOLE MEMBRANES; FILM NANOCOMPOSITE MEMBRANE; REVERSE-OSMOSIS SEPARATION; EXFOLIATED GRAPHITE OXIDE; NITRIC-ACID OXIDATION; CROSS-LINKING; ELECTROCHEMICAL REDUCTION; FUNCTIONALIZED GRAPHENE; COMPOSITE MEMBRANES;
D O I
10.1002/adfm.202006949
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Owing to the increasing need to mitigate excessive organic solvent waste, the efficient separation and recovery of organic solvents have received major research attention in recent years. The membrane-based organic solvent nanofiltration (OSN) process has demonstrated its feasibility in addressing this problem with low energy costs, compared to conventional separation techniques, such as adsorption, liquid-liquid extraction, and solvent evaporation. Recently, membranes made of 2D graphene-based materials have shown great promise because they attain high solvent flux and solute rejection using easy processing methods. Thus, this paper focuses on state-of-the-art studies of graphene-based membranes used in OSN processes, which include syntheses, characterizations, performance evaluations, membrane fouling, and simulation studies, in combination with the development of the "upper-bound" line to indicate the performance of graphene-based membranes. In this paper, critical challenges involved in the development of graphene-based membranes are also focused on and discussed to map out the future directions of these membranes in industrial OSN processes. In addition to OSN, this paper pertains to a broader audience in other separation processes, particularly in the fields of gas separation and water treatment.
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页数:36
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