Multi-heteroatom doped porous carbon derived from insect feces for capacitance-enhanced sodium-ion storage

被引：105
作者：
Chen, Chen [1 ]
Huang, Ying [1 ]
Meng, Zhuoyue [2 ]
Xu, Zhipeng [1 ]
Liu, Panbo [1 ]
Li, Tiehu [3 ]
机构：
[1] Northwestern Polytech Univ, Sch Chem & Chem Engn, MOE Key Lab Mat Phys & Chem Extraordinary Condit, Xian 710072, Shaanxi, Peoples R China
[2] Xian Univ Sci & Technol, Coll Chem & Chem Engn, Xian 710072, Shaanxi, Peoples R China
[3] Northwestern Polytech Univ, Shaanxi Joint Lab Graphene, Xian 710072, Shaanxi, Peoples R China
来源：
JOURNAL OF ENERGY CHEMISTRY | 2021年 / 54卷
基金：
中国国家自然科学基金;
关键词：
Heteroatom doped; Anode; Biomass; Sodium storage; Porous carbon; ELECTROCHEMICAL ENERGY-STORAGE; HARD CARBON; ANODE MATERIALS; NITROGEN; PERFORMANCE; OXYGEN; GRAPHENE; ROUTE;
D O I：
10.1016/j.jechem.2020.06.025
中图分类号：
O69 [应用化学];
学科分类号：
081704 ;
摘要：
The large-scale application of sodium ion batteries (SIBs) is limited by economic and environmental factors. Here, we prepare multi-heteroatom self-doped hierarchical porous carbon (HHPC) with a honeycomb-like structure by one-step carbonization method using high-yield and low-cost biomass silkworm excrement as a precursor. As an anode for SIB, HHPC-1100 exhibits a capacity of 331.7 mA h g(-1) at 20 mA g(-1), while it also reveals remarkable rate performance and stable long cycle capability due to its abundant pore structure and proper amount of hetero atom doping. Moreover, the synergistic effect of O, N, S, P co-doping in carbon materials on sodium ion adsorption is verified by the first-principles study, which provide a theoretical basis for the prominent electrochemical performance of the material. (C) 2020 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.
引用
收藏
页码：482 / 492
页数：11
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